Fix misalignment paragraph to extractions

bm_paragraph_level_no_spans_test.json

@@ -664,7 +664,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "9. Use of a filter press device for ternary precursor filtration washing according to claim 7, characterized in that: and in the second step, the sodium hydroxide solution is at the temperature of 60-80 \u2103 and the solute mass fraction is 1% -3%, and the pressure inside the filter press is 0.45-0.55MPa in the washing process of the alkali liquor and the washing process of the purified water.",
+        "paragraph": "2. The method for preparing the continuous nickel-cobalt-manganese ternary precursor according to claim 1, wherein the method comprises the following steps: the concentration of the ammonia water solution is 12-25 g/L.",
         "measurement_extractions": [
             {
                 "quantity": "12-25 g/L",
@@ -679,7 +679,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "2. The method for preparing the continuous nickel-cobalt-manganese ternary precursor according to claim 1, wherein the method comprises the following steps: the concentration of the ammonia water solution is 12-25 g/L.",
+        "paragraph": "14. The method of claim 9, wherein a pH of the first mixture in the first process is adjusted to be in a range of about 10 to about 11, and a pH of the second mixture in the second process is adjusted to be in a range of about 11.5 to about 12.0.",
         "measurement_extractions": [
             {
                 "quantity": "10 to about 11",
@@ -700,7 +700,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "7. The method for preparing the continuous nickel-cobalt-manganese ternary precursor according to claim 1, wherein the method comprises the following steps: and when the reaction is carried out in the reaction kettle, the temperature of the reaction kettle is controlled to be 40-80 \u2103, and the average residence time of the reaction liquid in the reaction kettle is 5-20 hours.",
+        "paragraph": "15. The method according to claim 13, wherein, in step 2, the inner cylinder was rotated at a speed of 10 to 5,000 rpm and the reactants are mixed at a temperature of 30 to 60\u00b0 C. and at a pH 10 to 12.",
         "measurement_extractions": [
             {
                 "quantity": "30 to 60\u00b0 C",
@@ -721,7 +721,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "14. The method of claim 9, wherein a pH of the first mixture in the first process is adjusted to be in a range of about 10 to about 11, and a pH of the second mixture in the second process is adjusted to be in a range of about 11.5 to about 12.0.",
+        "paragraph": "18. The method according to claim 13, wherein the aqueous ammonia solution is a 15 to 30% aqueous ammonia solution and is added at an amount of 1 to 20% by volume, with respect to the total weight of the mixed solution of the reactants.",
         "measurement_extractions": [
             {
                 "quantity": "1 to 20%",
@@ -736,7 +736,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "15. The method according to claim 13, wherein, in step 2, the inner cylinder was rotated at a speed of 10 to 5,000 rpm and the reactants are mixed at a temperature of 30 to 60\u00b0 C. and at a pH 10 to 12.",
+        "paragraph": "16. A positive electrode active material for nonaqueous electrolyte secondary batteries, the positive electrode active material comprising a lithium transition metal composite oxide represented by a general formula (2) Li1+uMxWsAtO2(wherein, \u22120.05\u2266u\u22660.50, x+s+t=1, 0<s\u22660.05, 0<s+t\u22660.15, M is at least one transition metal selected from Ni, Co and Mn, and A is at least one additive element selected from transition metal elements other than M and W, group 2 elements, and group 13 elements) and having a layered hexagonal crystal structure,wherein the positive electrode active material has an average particle diameter of 3 to 8 \u03bcm and an index indicating a scale of particle-size distribution, [(d90\u2212d10)/average-particle-diameter], of not more than 0.60.",
         "measurement_extractions": [
             {
                 "quantity": "3 to 8 \u03bcm",
@@ -757,7 +757,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "18. The method according to claim 13, wherein the aqueous ammonia solution is a 15 to 30% aqueous ammonia solution and is added at an amount of 1 to 20% by volume, with respect to the total weight of the mixed solution of the reactants.",
+        "paragraph": "17. The positive electrode active material for nonaqueous electrolyte secondary batteries according toclaim 16, wherein a specific surface area is 0.5 to 2.0 m2/g.",
         "measurement_extractions": [
             {
                 "quantity": "0.5 to 2.0 m2/g",
@@ -772,7 +772,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "16. A positive electrode active material for nonaqueous electrolyte secondary batteries, the positive electrode active material comprising a lithium transition metal composite oxide represented by a general formula (2) Li1+uMxWsAtO2(wherein, \u22120.05\u2266u\u22660.50, x+s+t=1, 0<s\u22660.05, 0<s+t\u22660.15, M is at least one transition metal selected from Ni, Co and Mn, and A is at least one additive element selected from transition metal elements other than M and W, group 2 elements, and group 13 elements) and having a layered hexagonal crystal structure,wherein the positive electrode active material has an average particle diameter of 3 to 8 \u03bcm and an index indicating a scale of particle-size distribution, [(d90\u2212d10)/average-particle-diameter], of not more than 0.60.",
+        "paragraph": "8. A transition metal composite hydroxide represented by a general formula (1) MxWsAt(OH)2+\u03b1(wherein, x+s+t=1, 0<s\u22660.05, 0<s+t\u22660.15, 0\u2266\u03b1\u22660.5, M is at least one transition metal selected from Ni, Co and Mn, and A is at least one additive element selected from transition metal elements other than M and W, group 2 elements, and group 13 elements) and serving as a precursor of a positive electrode active material for nonaqueous electrolyte secondary batteries, whereinthe transition metal composite hydroxide is a secondary particle having a substantially spherical shape and composed of aggregation of a plurality of primary particles,the secondary particle has an average particle diameter of 3 to 7 \u03bcm and an index indicating a scale of particle-size distribution, [(d90\u2212d10)/average-particle-diameter], of not more than 0.55, anda coating material containing a metal oxide of tungsten and the additive element or a metal hydroxide of tungsten and the additive element is formed on surfaces of the secondary particles.\nthe transition metal composite hydroxide is a secondary particle having a substantially spherical shape and composed of aggregation of a plurality of primary particles,\nthe secondary particle has an average particle diameter of 3 to 7 \u03bcm and an index indicating a scale of particle-size distribution, [(d90\u2212d10)/average-particle-diameter], of not more than 0.55, and\na coating material containing a metal oxide of tungsten and the additive element or a metal hydroxide of tungsten and the additive element is formed on surfaces of the secondary particles.",
         "measurement_extractions": [
             {
                 "quantity": "3 to 7 \u03bcm",
@@ -793,7 +793,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "17. The positive electrode active material for nonaqueous electrolyte secondary batteries according toclaim 16, wherein a specific surface area is 0.5 to 2.0 m2/g.",
+        "paragraph": "9. The transition metal composite hydroxide according toclaim 8, wherein a specific surface area is 5 to 30 m2/g.",
         "measurement_extractions": [
             {
                 "quantity": "5 to 30 m2/g",
@@ -808,7 +808,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "8. A transition metal composite hydroxide represented by a general formula (1) MxWsAt(OH)2+\u03b1(wherein, x+s+t=1, 0<s\u22660.05, 0<s+t\u22660.15, 0\u2266\u03b1\u22660.5, M is at least one transition metal selected from Ni, Co and Mn, and A is at least one additive element selected from transition metal elements other than M and W, group 2 elements, and group 13 elements) and serving as a precursor of a positive electrode active material for nonaqueous electrolyte secondary batteries, whereinthe transition metal composite hydroxide is a secondary particle having a substantially spherical shape and composed of aggregation of a plurality of primary particles,the secondary particle has an average particle diameter of 3 to 7 \u03bcm and an index indicating a scale of particle-size distribution, [(d90\u2212d10)/average-particle-diameter], of not more than 0.55, anda coating material containing a metal oxide of tungsten and the additive element or a metal hydroxide of tungsten and the additive element is formed on surfaces of the secondary particles.\nthe transition metal composite hydroxide is a secondary particle having a substantially spherical shape and composed of aggregation of a plurality of primary particles,\nthe secondary particle has an average particle diameter of 3 to 7 \u03bcm and an index indicating a scale of particle-size distribution, [(d90\u2212d10)/average-particle-diameter], of not more than 0.55, and\na coating material containing a metal oxide of tungsten and the additive element or a metal hydroxide of tungsten and the additive element is formed on surfaces of the secondary particles.",
+        "paragraph": "What is claimed is:\n1. A nickel composite hydroxide, comprising:\na composition represented by Ni<sub>1-x-y-z </sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>(OH)<sub>2+A </sub>(where 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, 0\u2266A\u22660.5, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W),\nwherein the nickel composite hydroxide is composed of secondary particles in which spherical or lump-shaped nickel composite hydroxide particles, which are formed by a plurality of primary particles aggregated with one after another, are coupled with one after another in two dimensional directions, and\nwherein the secondary particles have a volume average particle size (Mv) of 4 to 20 \u03bcm measured by a laser diffraction/scattering method and a ratio (Mv/L) of the volume average particle size relative to the width (L) of the secondary particles in a direction perpendicular to the coupling direction of the nickel composite hydroxide particles in a range from 3 to 20.",
         "measurement_extractions": [
             {
                 "quantity": "4 to 20 \u03bcm",
@@ -823,7 +823,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "9. The transition metal composite hydroxide according toclaim 8, wherein a specific surface area is 5 to 30 m2/g.",
+        "paragraph": "11. A positive electrode active material for a nonaqueous electrolytic secondary cell composed of a lithium nickel composite oxide represented by Li<sub>1+u</sub>Ni<sub>1-x-y-z</sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>O<sub>2 </sub>(where, \u22120.05\u2266u\u22660.50, 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W),\nwherein the lithium nickel composite oxide is composed of secondary particles in which spherical or lump-shaped lithium nickel composite hydroxide particles, which are formed by a plurality of primary particles aggregated with one after another, are coupled with one after another in two-dimensional directions, and\nwherein the secondary particles have a volume average particle size (Mv) of 4 to 20 \u03bcm measured by a laser diffraction/scattering method and a ratio (Mv/L) of the volume average particle size relative to the width (L) of the secondary particles in a direction perpendicular to the coupling direction of the nickel composite hydroxide particles in a range from 3 to 20.",
         "measurement_extractions": [
             {
                 "quantity": "4 to 20 \u03bcm",
@@ -838,7 +838,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "What is claimed is:\n1. A nickel composite hydroxide, comprising:\na composition represented by Ni<sub>1-x-y-z </sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>(OH)<sub>2+A </sub>(where 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, 0\u2266A\u22660.5, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W),\nwherein the nickel composite hydroxide is composed of secondary particles in which spherical or lump-shaped nickel composite hydroxide particles, which are formed by a plurality of primary particles aggregated with one after another, are coupled with one after another in two dimensional directions, and\nwherein the secondary particles have a volume average particle size (Mv) of 4 to 20 \u03bcm measured by a laser diffraction/scattering method and a ratio (Mv/L) of the volume average particle size relative to the width (L) of the secondary particles in a direction perpendicular to the coupling direction of the nickel composite hydroxide particles in a range from 3 to 20.",
+        "paragraph": "12. The positive electrode active material according to claim 11, further comprising:\na specific surface area in a range from 0.3 to 2 m2/g.",
         "measurement_extractions": [
             {
                 "quantity": "from 0.3 to 2 m2/g",
@@ -853,7 +853,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "11. A positive electrode active material for a nonaqueous electrolytic secondary cell composed of a lithium nickel composite oxide represented by Li<sub>1+u</sub>Ni<sub>1-x-y-z</sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>O<sub>2 </sub>(where, \u22120.05\u2266u\u22660.50, 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W),\nwherein the lithium nickel composite oxide is composed of secondary particles in which spherical or lump-shaped lithium nickel composite hydroxide particles, which are formed by a plurality of primary particles aggregated with one after another, are coupled with one after another in two-dimensional directions, and\nwherein the secondary particles have a volume average particle size (Mv) of 4 to 20 \u03bcm measured by a laser diffraction/scattering method and a ratio (Mv/L) of the volume average particle size relative to the width (L) of the secondary particles in a direction perpendicular to the coupling direction of the nickel composite hydroxide particles in a range from 3 to 20.",
+        "paragraph": "13. The positive electrode active material according to claim 11, wherein the positive electrode active material has a deviation index [(D90\u2212D10)/Mv] of particle size of 0.75 or less, which is calculated by using D90 and D10 in grain size distribution obtained by a laser diffraction/scattering method and the volume average particle size (Mv).",
         "measurement_extractions": [
             {
                 "quantity": "0.75 or less",
@@ -868,7 +868,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "12. The positive electrode active material according to claim 11, further comprising:\na specific surface area in a range from 0.3 to 2 m2/g.",
+        "paragraph": "17. A method of producing a positive electrode active material for a nonaqueous electrolytic secondary cell composed of a lithium nickel composite oxide represented by Li<sub>1+u</sub>Ni<sub>1-x-y-z </sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>O<sub>2 </sub>(where, \u22120.05\u2266u\u22660.50, 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W), comprising the steps of:\nmixing the nickel composite hydroxide according to claim 1 with a lithium compound so that a lithium mixed material is formed; and\nbaking the lithium mixed material produced in the mixing step in an oxidizing atmosphere at a temperature of 650\u00b0 C. to 980\u00b0 C.",
         "measurement_extractions": [
             {
                 "quantity": "650\u00b0 C. to 980\u00b0 C",
@@ -883,7 +883,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "13. The positive electrode active material according to claim 11, wherein the positive electrode active material has a deviation index [(D90\u2212D10)/Mv] of particle size of 0.75 or less, which is calculated by using D90 and D10 in grain size distribution obtained by a laser diffraction/scattering method and the volume average particle size (Mv).",
+        "paragraph": "19. The method of producing a positive electrode active material according to claim 17, further comprising the step of:\nprior to the mixing step, carrying out a thermal treatment on the nickel composite hydroxide at a temperature of 300 to 750\u00b0 C. in a non-reducing atmosphere or in an air flow.",
         "measurement_extractions": [
             {
                 "quantity": "300 to 750\u00b0 C",
@@ -898,7 +898,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "17. A method of producing a positive electrode active material for a nonaqueous electrolytic secondary cell composed of a lithium nickel composite oxide represented by Li<sub>1+u</sub>Ni<sub>1-x-y-z </sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>O<sub>2 </sub>(where, \u22120.05\u2266u\u22660.50, 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W), comprising the steps of:\nmixing the nickel composite hydroxide according to claim 1 with a lithium compound so that a lithium mixed material is formed; and\nbaking the lithium mixed material produced in the mixing step in an oxidizing atmosphere at a temperature of 650\u00b0 C. to 980\u00b0 C.",
+        "paragraph": "2. The nickel composite hydroxide according to claim 1, wherein the nickel composite hydroxide has a deviation index [(D90\u2212D10)/Mv] of particle size of 0.70 or less, which is calculated by using D90 and D10 in grain size distribution obtained by a laser diffraction/scattering method and a volume average particle size (Mv).",
         "measurement_extractions": [
             {
                 "quantity": "0.70 or less",
@@ -913,7 +913,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "19. The method of producing a positive electrode active material according to claim 17, further comprising the step of:\nprior to the mixing step, carrying out a thermal treatment on the nickel composite hydroxide at a temperature of 300 to 750\u00b0 C. in a non-reducing atmosphere or in an air flow.",
+        "paragraph": "6. A method of producing a nickel composite hydroxide represented by: Ni<sub>1-x-y-z</sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>(OH)<sub>2+A </sub>(where 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, 0\u2266A\u22660.5, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W), comprising the steps of:\ngenerating a plate-shaped crystal core by allowing a crystal core generating aqueous solution composed of a metal compound aqueous solution containing cobalt and/or manganese to have a pH value of 7.5 to 11.1 at a standard liquid temperature of 25\u00b0 C.; and\nsetting a pH value of slurry for a particle growth containing the plate-shaped crystal core generated in the crystal core generating step to 10.5 to 12.5 at a standard liquid temperature of 25\u00b0 C., while supplying a mixed aqueous solution including a metal compound containing at least nickel to slurry for the particle growth so that the plate-shaped crystal core is grown as particles.",
         "measurement_extractions": [
             {
                 "quantity": "7.5 to 11.1",
@@ -946,7 +946,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "2. The nickel composite hydroxide according to claim 1, wherein the nickel composite hydroxide has a deviation index [(D90\u2212D10)/Mv] of particle size of 0.70 or less, which is calculated by using D90 and D10 in grain size distribution obtained by a laser diffraction/scattering method and a volume average particle size (Mv).",
+        "paragraph": "8. The method of producing a nickel composite hydroxide according to claim 6, wherein in the particle growing step, slurry for the particle growth has an ammonia concentration of 5 to 20 g/l.",
         "measurement_extractions": [
             {
                 "quantity": "5 to 20 g/l",
@@ -961,7 +961,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "6. A method of producing a nickel composite hydroxide represented by: Ni<sub>1-x-y-z</sub>Co<sub>x</sub>Mn<sub>y</sub>M<sub>z</sub>(OH)<sub>2+A </sub>(where 0\u2266x\u22660.35, 0\u2266y\u22660.35, 0\u2266z\u22660.1, 0<x+y, 0<x+y+z\u22660.7, 0\u2266A\u22660.5, with M being at least one kind of additive element selected from the group consisting of V, Mg, Al, Ti, Mo, Nb, Zr and W), comprising the steps of:\ngenerating a plate-shaped crystal core by allowing a crystal core generating aqueous solution composed of a metal compound aqueous solution containing cobalt and/or manganese to have a pH value of 7.5 to 11.1 at a standard liquid temperature of 25\u00b0 C.; and\nsetting a pH value of slurry for a particle growth containing the plate-shaped crystal core generated in the crystal core generating step to 10.5 to 12.5 at a standard liquid temperature of 25\u00b0 C., while supplying a mixed aqueous solution including a metal compound containing at least nickel to slurry for the particle growth so that the plate-shaped crystal core is grown as particles.",
+        "paragraph": "What is claimed is:\n1. A lithium-rich lithium metal complex oxide containing at least 50 mol % of Mn with respect to a total amount of metals other than lithium, and at least one other metal, the lithium metal complex oxide having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
         "measurement_extractions": [
             {
                 "quantity": "1.0 g/ml to 2.0 g/ml",
@@ -976,7 +976,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "8. The method of producing a nickel composite hydroxide according to claim 6, wherein in the particle growing step, slurry for the particle growth has an ammonia concentration of 5 to 20 g/l.",
+        "paragraph": "3. The lithium metal complex oxide according to claim 1, wherein an average particle diameter (D50) is in a range of 1 \u03bcm to 10 \u03bcm.",
         "measurement_extractions": [
             {
                 "quantity": "1 \u03bcm to 10 \u03bcm",
@@ -991,7 +991,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "What is claimed is:\n1. A lithium-rich lithium metal complex oxide containing at least 50 mol % of Mn with respect to a total amount of metals other than lithium, and at least one other metal, the lithium metal complex oxide having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
+        "paragraph": "6. The lithium metal complex oxide according to claim 1, obtained by baking a metal complex hydroxide with a lithium compound, the metal complex hydroxide being obtained by a coprecipitation process carried out without a complexing agent and containing at least 50 mol % of Mn with respect to a total amount of metals, and at least one other metal, and having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
         "measurement_extractions": [
             {
                 "quantity": "1.0 g/ml to 2.0 g/ml",
@@ -1006,7 +1006,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "3. The lithium metal complex oxide according to claim 1, wherein an average particle diameter (D50) is in a range of 1 \u03bcm to 10 \u03bcm.",
+        "paragraph": "7. A method of producing the lithium metal complex oxide of claim 1, comprising:\nbaking a metal complex hydroxide with a lithium compound, the metal complex hydroxide being obtained by a coprecipitation process carried out without a complexing agent and containing at least 50 mol % of Mn with respect to a total amount of metals, and at least one other metal, and having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
         "measurement_extractions": [
             {
                 "quantity": "1.0 g/ml to 2.0 g/ml",
@@ -1021,7 +1021,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "6. The lithium metal complex oxide according to claim 1, obtained by baking a metal complex hydroxide with a lithium compound, the metal complex hydroxide being obtained by a coprecipitation process carried out without a complexing agent and containing at least 50 mol % of Mn with respect to a total amount of metals, and at least one other metal, and having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
+        "paragraph": "9. A metal complex hydroxide obtained by a coprecipitation process carried out without a complexing agent and containing at least 50 mol % of Mn with respect to a total amount of metals, and at least one other metal, and having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
         "measurement_extractions": [
             {
                 "quantity": "1.0 g/ml to 2.0 g/ml",
@@ -1036,7 +1036,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "7. A method of producing the lithium metal complex oxide of claim 1, comprising:\nbaking a metal complex hydroxide with a lithium compound, the metal complex hydroxide being obtained by a coprecipitation process carried out without a complexing agent and containing at least 50 mol % of Mn with respect to a total amount of metals, and at least one other metal, and having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
+        "paragraph": "1. Precursor particles of a lithium composite transition metal oxide for lithium secondary batteries, wherein the precursor particles are composite transition metal hydroxide particles comprising at least two transition metals and having an average diameter of 1 \u03bcm to 8 \u03bcm, wherein the composite transition metal hydroxide particles exhibit monodisperse particle size distribution and have a coefficient of variation of 0.2 to 0.7.",
         "measurement_extractions": [
             {
                 "quantity": "1 \u03bcm to 8 \u03bcm",
@@ -1051,7 +1051,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "9. A metal complex hydroxide obtained by a coprecipitation process carried out without a complexing agent and containing at least 50 mol % of Mn with respect to a total amount of metals, and at least one other metal, and having a tapped density in a range of 1.0 g/ml to 2.0 g/ml.",
+        "paragraph": "11. Lithium composite transition metal oxide particles comprising at least two transition metals and having an average diameter of 1.0 \u03bcm to 8.5 \u03bcm, wherein the lithium composite transition metal oxide particles exhibit monodisperse particle size distribution and have a coefficient of variation of 0.2 to 0.7.",
         "measurement_extractions": [
             {
                 "quantity": "1.0 \u03bcm to 8.5 \u03bcm",
@@ -1066,7 +1066,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "1. Precursor particles of a lithium composite transition metal oxide for lithium secondary batteries, wherein the precursor particles are composite transition metal hydroxide particles comprising at least two transition metals and having an average diameter of 1 \u03bcm to 8 \u03bcm, wherein the composite transition metal hydroxide particles exhibit monodisperse particle size distribution and have a coefficient of variation of 0.2 to 0.7.",
+        "paragraph": "12. The lithium composite transition metal oxide particles according toclaim 11, wherein the average diameter of the lithium composite transition metal oxide particles is 1.0 \u03bcm to 5.5 \u03bcm.",
         "measurement_extractions": [
             {
                 "quantity": "1.0 \u03bcm to 5.5 \u03bcm",
@@ -1081,7 +1081,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "11. Lithium composite transition metal oxide particles comprising at least two transition metals and having an average diameter of 1.0 \u03bcm to 8.5 \u03bcm, wherein the lithium composite transition metal oxide particles exhibit monodisperse particle size distribution and have a coefficient of variation of 0.2 to 0.7.",
+        "paragraph": "2. The precursor particles according toclaim 1, wherein the average diameter of the composite transition metal hydroxide particles is 1 \u03bcm to 5 \u03bcm.",
         "measurement_extractions": [
             {
                 "quantity": "1 \u03bcm to 5 \u03bcm",
@@ -1096,7 +1096,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "12. The lithium composite transition metal oxide particles according toclaim 11, wherein the average diameter of the lithium composite transition metal oxide particles is 1.0 \u03bcm to 5.5 \u03bcm.",
+        "paragraph": "2. The active material precursor of claim 1, wherein a tap density of the active material precursor is about 1.95 g/ml or lower.",
         "measurement_extractions": [
             {
                 "quantity": "1.95 g/ml or lower",
@@ -1111,7 +1111,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "2. The precursor particles according toclaim 1, wherein the average diameter of the composite transition metal hydroxide particles is 1 \u03bcm to 5 \u03bcm.",
+        "paragraph": "6. A method of preparing the active material precursor of claim 1, the method comprising:\nmixing a nickel precursor, a manganese precursor, a cobalt precursor, a metal (M) precursor, and a solvent to prepare a precursor mixture; and\nmixing the precursor mixture and a pH adjusting agent to adjust a pH value of the resultant to be in a range of about 11.0 to about 11.2.",
         "measurement_extractions": [
             {
                 "quantity": "11.0 to about 11.2",
@@ -1126,7 +1126,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "2. The active material precursor of claim 1, wherein a tap density of the active material precursor is about 1.95 g/ml or lower.",
+        "paragraph": "1. A method for preparing transition metal composite hydroxide particles using a reactor having a closed structure, the method comprising:injecting raw materials comprising an aqueous solution of two or more transition metal salts and an aqueous solution of a complex-forming additive, and a basic aqueous solution for maintaining pH of an aqueous solution of the raw materials within a range of 10 to 12, into the rotation reaction area of the reactor through the inlet; andperforming coprecipitation reaction under a non-nitrogen atmosphere for 1 to 6 hours,wherein the reactor comprises:a stationary hollow cylinder;a rotary cylinder having the same axis as the stationary hollow cylinder and an outer diameter smaller than an inner diameter of the stationary hollow cylinder;an electric motor to generate power, enabling rotation of the rotary cylinder;a rotation reaction area disposed between the stationary hollow cylinder and the rotary cylinder, wherein ring-shaped vortex pairs that are uniformly arranged in a rotation axis direction and rotate in opposite directions are formed in the rotation reaction area; andan inlet through which a reactant fluid is fed into the rotation reaction area and an outlet through which the reactant fluid is discharged from the rotation reaction area,wherein a ratio of a distance between the stationary hollow cylinder and the rotary cylinder to the outer radius of the rotary cylinder is higher than 0.05 and lower than 0.4.",
         "measurement_extractions": [
             {
                 "quantity": "10 to 12",
@@ -1141,7 +1141,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "6. A method of preparing the active material precursor of claim 1, the method comprising:\nmixing a nickel precursor, a manganese precursor, a cobalt precursor, a metal (M) precursor, and a solvent to prepare a precursor mixture; and\nmixing the precursor mixture and a pH adjusting agent to adjust a pH value of the resultant to be in a range of about 11.0 to about 11.2.",
+        "paragraph": "10. A positive electrode active material for nonaqueous electrolyte secondary batteries, comprising a lithium-transition metal composite oxide represented by a general formula LidNi1\u2212a\u2212b\u2212cCoaMbNbcO2where 0.03\u2266a\u22660.35; 0\u2266b\u22660.10; 0.001\u2266c\u22660.05; 0.95\u2266d\u22661.20; and M is at least one element selected from Mn, V, Mg, Ti, and Al and consisting of particles of polycrystalline structure, whereina specific surface area of the positive electrode active material is 0.9 to 4.0 m2/g,a crystallite diameter of the positive electrode active material is 10 to 150 nm, anda content of alkali metals other than lithium is 20 mass ppm or less.\na specific surface area of the positive electrode active material is 0.9 to 4.0 m2/g,\na crystallite diameter of the positive electrode active material is 10 to 150 nm, and\na content of alkali metals other than lithium is 20 mass ppm or less.",
         "measurement_extractions": [
             {
                 "quantity": "0.9 to 4.0 m2/g",
@@ -1156,7 +1156,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "1. A method for preparing transition metal composite hydroxide particles using a reactor having a closed structure, the method comprising:injecting raw materials comprising an aqueous solution of two or more transition metal salts and an aqueous solution of a complex-forming additive, and a basic aqueous solution for maintaining pH of an aqueous solution of the raw materials within a range of 10 to 12, into the rotation reaction area of the reactor through the inlet; andperforming coprecipitation reaction under a non-nitrogen atmosphere for 1 to 6 hours,wherein the reactor comprises:a stationary hollow cylinder;a rotary cylinder having the same axis as the stationary hollow cylinder and an outer diameter smaller than an inner diameter of the stationary hollow cylinder;an electric motor to generate power, enabling rotation of the rotary cylinder;a rotation reaction area disposed between the stationary hollow cylinder and the rotary cylinder, wherein ring-shaped vortex pairs that are uniformly arranged in a rotation axis direction and rotate in opposite directions are formed in the rotation reaction area; andan inlet through which a reactant fluid is fed into the rotation reaction area and an outlet through which the reactant fluid is discharged from the rotation reaction area,wherein a ratio of a distance between the stationary hollow cylinder and the rotary cylinder to the outer radius of the rotary cylinder is higher than 0.05 and lower than 0.4.",
+        "paragraph": "11. The positive electrode active material for nonaqueous electrolyte secondary batteries ofclaim 23, wherein the specific surface area of the positive electrode active material is 0.9 to 3.0 m2/g.",
         "measurement_extractions": [
             {
                 "quantity": "0.9 to 3.0 m2/g",
@@ -1171,7 +1171,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "10. A positive electrode active material for nonaqueous electrolyte secondary batteries, comprising a lithium-transition metal composite oxide represented by a general formula LidNi1\u2212a\u2212b\u2212cCoaMbNbcO2where 0.03\u2266a\u22660.35; 0\u2266b\u22660.10; 0.001\u2266c\u22660.05; 0.95\u2266d\u22661.20; and M is at least one element selected from Mn, V, Mg, Ti, and Al and consisting of particles of polycrystalline structure, whereina specific surface area of the positive electrode active material is 0.9 to 4.0 m2/g,a crystallite diameter of the positive electrode active material is 10 to 150 nm, anda content of alkali metals other than lithium is 20 mass ppm or less.\na specific surface area of the positive electrode active material is 0.9 to 4.0 m2/g,\na crystallite diameter of the positive electrode active material is 10 to 150 nm, and\na content of alkali metals other than lithium is 20 mass ppm or less.",
+        "paragraph": "2. A method for producing a positive electrode active material for nonaqueous electrolyte secondary batteries, the positive electrode active material comprising a lithium-transition metal composite oxide represented by a general formula LidNi1\u2212a\u2212b\u2212cMbNbcO2where 0.03\u2266a\u22660.35; 0\u2266b\u22660.10; 0.001\u2266c\u22660.05; 0.95\u2266d\u22661.20; and M is at least one element selected from Mn, V, Mg, Ti, and Al and consisting of porous particles, the method comprising:a crystallization step of adding an alkaline aqueous solution to a mixed aqueous solution containing at least nickel and cobalt for crystallization to obtain a nickel-containing hydroxide represented by a general formula Ni1\u2212a\u2032\u2212b\u2032Coa\u2032Mb\u2032(OH)2where 0.03\u2266a\u2032\u22660.35; 0\u2266b\u2032\u22660.10; and M is at least one element selected from Mn, V, Mg, Ti, and Al;a mixing step of mixing the nickel-containing hydroxide, a lithium compound, and a niobium compound having an average particle diameter of 0.1 to 10 \u03bcm to obtain a lithium mixture; anda firing step of firing the lithium mixture in an oxidative atmosphere at 700 to 840\u00b0 C. to obtain the lithium-transition metal composite oxide.",
         "measurement_extractions": [
             {
                 "quantity": "0.1 to 10 \u03bcm",
@@ -1186,7 +1186,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "11. The positive electrode active material for nonaqueous electrolyte secondary batteries ofclaim 23, wherein the specific surface area of the positive electrode active material is 0.9 to 3.0 m2/g.",
+        "paragraph": "5. The method for producing a positive electrode active material for nonaqueous electrolyte secondary batteries ofclaim 15, further comprising a heat treatment step of, prior to the mixing step, heat-treating the nickel-containing hydroxide at a temperature of 105 to 800\u00b0 C., whereinthe mixing step comprises mixing a nickel-containing hydroxide and/or a nickel-containing oxide obtained in the heat treatment step, the lithium, compound, and the niobiumn compound to obtain a lithium mixture.\nthe mixing step comprises mixing a nickel-containing hydroxide and/or a nickel-containing oxide obtained in the heat treatment step, the lithium, compound, and the niobiumn compound to obtain a lithium mixture.",
         "measurement_extractions": [
             {
                 "quantity": "105 to 800\u00b0 C.",
@@ -1201,7 +1201,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "2. A method for producing a positive electrode active material for nonaqueous electrolyte secondary batteries, the positive electrode active material comprising a lithium-transition metal composite oxide represented by a general formula LidNi1\u2212a\u2212b\u2212cMbNbcO2where 0.03\u2266a\u22660.35; 0\u2266b\u22660.10; 0.001\u2266c\u22660.05; 0.95\u2266d\u22661.20; and M is at least one element selected from Mn, V, Mg, Ti, and Al and consisting of porous particles, the method comprising:a crystallization step of adding an alkaline aqueous solution to a mixed aqueous solution containing at least nickel and cobalt for crystallization to obtain a nickel-containing hydroxide represented by a general formula Ni1\u2212a\u2032\u2212b\u2032Coa\u2032Mb\u2032(OH)2where 0.03\u2266a\u2032\u22660.35; 0\u2266b\u2032\u22660.10; and M is at least one element selected from Mn, V, Mg, Ti, and Al;a mixing step of mixing the nickel-containing hydroxide, a lithium compound, and a niobium compound having an average particle diameter of 0.1 to 10 \u03bcm to obtain a lithium mixture; anda firing step of firing the lithium mixture in an oxidative atmosphere at 700 to 840\u00b0 C. to obtain the lithium-transition metal composite oxide.",
+        "paragraph": "1. A method of making a powder comprising a partly oxidized mixed metal hydroxide as a precursor for the preparation of cathode material for lithium secondary batteries,the partly oxidized mixed metal hydroxide being a homogeneous product represented by the formulaNibM1cM2d(O)x(OH)ywhereinM1 denotes only one element selected from the group consisting of Fe, Co, Mg, Zn, and Cu,M2 denotes only one element selected from the group consisting of Mn, B, and Cr,b\u22660.8c\u22660.5d\u22660.5, andx is a number between 0.1 and 0.54,y is a number between 1.46 and 1.9, and x+y=2, which has an average degree of oxidation of 2.1 to 2.54, andwherein the partly oxidized mixed metal hydroxide further contains sodium, and a content of sodium in the partly oxidized mixed metal hydroxide is less than 2,000 ppm, and wherein the powder has a standardized width of a particle size distribution, defined according to formula (1), is less than 1.8(D90\u2212D10)/D50 \u2003\u2003(1),wherein D denotes a diameter of the powder particles, andwherein the powder has an average particle size, measured in accordance with ASTM B 822, of 2-30 \u03bcmthe method comprising the following steps:a. co-precipitating spherical mixed metal hydroxides from corresponding metal salt solutions,b. separating off the co-precipitated mixed metal hydroxide from the suspension,c. washing the mixed metal hydroxide,d. drying and simultaneously partially oxidizing the mixed metal hydroxide under an oxygen-containing atmosphere at a temperature of greater than 80\u00b0 C. for at least 3 hours.",
         "measurement_extractions": [
             {
                 "quantity": "less than 2,000 ppm",
@@ -1228,7 +1228,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "5. The method for producing a positive electrode active material for nonaqueous electrolyte secondary batteries ofclaim 15, further comprising a heat treatment step of, prior to the mixing step, heat-treating the nickel-containing hydroxide at a temperature of 105 to 800\u00b0 C., whereinthe mixing step comprises mixing a nickel-containing hydroxide and/or a nickel-containing oxide obtained in the heat treatment step, the lithium, compound, and the niobiumn compound to obtain a lithium mixture.\nthe mixing step comprises mixing a nickel-containing hydroxide and/or a nickel-containing oxide obtained in the heat treatment step, the lithium, compound, and the niobiumn compound to obtain a lithium mixture.",
+        "paragraph": "5. The method according toclaim 1, wherein the content of sodium in the partly oxidized mixed metal hydroxide is less than 1,000 ppm.",
         "measurement_extractions": [
             {
                 "quantity": "less than 1,000 ppm",

bm_paragraph_level_no_spans_train.json

@@ -2914,7 +2914,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "1. A method of preparing a positive electrode active material precursor for a lithium secondary battery comprising:adding a reaction solution including a first transition metal-containing solution, a second transition metal-containing solution, an ammonium ion-containing solution, and a basic aqueous solution to a batch reactor, wherein the adding of the reaction solution is done while continuously discharging a portion of the reaction solution in the batch reactor to outside of the batch reactor when the batch reactor is full,wherein an initial input flow rate of the reaction solution added to the batch reactor satisfies following Equation 1, anda pH in the batch reactor satisfies following Equation 2:1.5\u00d7V/t\u2264\u03c51+\u03c52+\u03c53\u226410\u00d7V/t[Equation 1]wherein, in Equation 1,V is a volume of the batch reactor, t is total reaction time (minutes), \u03c51is a total initial input flow rate (mL/min) of the first transition metal-containing solution and the second transition metal-containing solution, \u03c52is an initial input flow rate (mL/min) of the ammonium ion-containing solution, and \u03c53is an initial input flow rate (mL/min) of the basic aqueous solution, andpH0\u2212{([Ni]0\u2212[Ni]t1)\u00d70.05}\u2264pHt1\u2264pH0\u2212{([Ni]0\u2212[Ni]t1)\u00d70.005}\u2003\u2003[Equation 2]wherein, in Equation 2,pHt1is a pH in the batch reactor at time t1, pH0is an initial pH in the batch reactor, [Ni]0is a molar concentration of nickel (Ni) in the transition metal-containing solution initially added, and [Ni]t1is a molar concentration of Ni in the transition metal-containing solution added at time t1.\nadding a reaction solution including a first transition metal-containing solution, a second transition metal-containing solution, an ammonium ion-containing solution, and a basic aqueous solution to a batch reactor, wherein the adding of the reaction solution is done while continuously discharging a portion of the reaction solution in the batch reactor to outside of the batch reactor when the batch reactor is full,\nwherein an initial input flow rate of the reaction solution added to the batch reactor satisfies following Equation 1, and\na pH in the batch reactor satisfies following Equation 2:1.5\u00d7V/t\u2264\u03c51+\u03c52+\u03c53\u226410\u00d7V/t[Equation 1]\n1.5\u00d7V/t\u2264\u03c51+\u03c52+\u03c53\u226410\u00d7V/t[Equation 1]\nwherein, in Equation 1,\nV is a volume of the batch reactor, t is total reaction time (minutes), \u03c51is a total initial input flow rate (mL/min) of the first transition metal-containing solution and the second transition metal-containing solution, \u03c52is an initial input flow rate (mL/min) of the ammonium ion-containing solution, and \u03c53is an initial input flow rate (mL/min) of the basic aqueous solution, andpH0\u2212{([Ni]0\u2212[Ni]t1)\u00d70.05}\u2264pHt1\u2264pH0\u2212{([Ni]0\u2212[Ni]t1)\u00d70.005}\u2003\u2003[Equation 2]\npH0\u2212{([Ni]0\u2212[Ni]t1)\u00d70.05}\u2264pHt1\u2264pH0\u2212{([Ni]0\u2212[Ni]t1)\u00d70.005}\u2003\u2003[Equation 2]\nwherein, in Equation 2,\npHt1is a pH in the batch reactor at time t1, pH0is an initial pH in the batch reactor, [Ni]0is a molar concentration of nickel (Ni) in the transition metal-containing solution initially added, and [Ni]t1is a molar concentration of Ni in the transition metal-containing solution added at time t1.",
+        "paragraph": "11. The active material of claim 1, wherein the active material precursor is obtained by a method comprising:\nmixing a nickel precursor, a manganese precursor, a cobalt precursor, a metal (M) precursor, and a solvent to prepare a precursor mixture; and\nmixing the precursor mixture and a pH adjusting agent to adjust a pH value of the resultant to be in a range of about 11.0 to about 11.2.",
         "measurement_extractions": [
             {
                 "quantity": "range of about 11.0 to about 11.2",
@@ -2929,7 +2929,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "11. The active material of claim 1, wherein the active material precursor is obtained by a method comprising:\nmixing a nickel precursor, a manganese precursor, a cobalt precursor, a metal (M) precursor, and a solvent to prepare a precursor mixture; and\nmixing the precursor mixture and a pH adjusting agent to adjust a pH value of the resultant to be in a range of about 11.0 to about 11.2.",
+        "paragraph": "4. The active material precursor of claim 1, wherein a tap density of the active material precursor is about 1.95 g/ml or lower.",
         "measurement_extractions": [
             {
                 "quantity": "1.95 g/ml",
@@ -2944,7 +2944,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "4. The active material precursor of claim 1, wherein a tap density of the active material precursor is about 1.95 g/ml or lower.",
+        "paragraph": "13. A positive electrode active material for a non-aqueous electrolyte secondary battery which includes secondary particles formed by aggregates of a plurality of primary particles and having a tap density of 1.5 g/cm3or more and a surface roughness index which is a value in which the measured specific surface area of the secondary particles is divided by the geometric surface area of the secondary particles when the secondary particles are assumed to be true sphere is within a range of 3.6 to 10.",
         "measurement_extractions": [
             {
                 "quantity": "1.5 g/cm3",
@@ -2959,7 +2959,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "13. A positive electrode active material for a non-aqueous electrolyte secondary battery which includes secondary particles formed by aggregates of a plurality of primary particles and having a tap density of 1.5 g/cm3or more and a surface roughness index which is a value in which the measured specific surface area of the secondary particles is divided by the geometric surface area of the secondary particles when the secondary particles are assumed to be true sphere is within a range of 3.6 to 10.",
+        "paragraph": "14. The positive electrode active material for a non-aqueous electrolyte secondary battery according to claim 13, wherein the average particle size of the secondary particles is within a range of 1 \u03bcm to 15 \u03bcm, and the value of [(d90\u2212d10)/average particle size], which is an index indicating the spread of the particle size distribution of the secondary particles, is 0.7 or less.",
         "measurement_extractions": [
             {
                 "quantity": "a range of 1 \u03bcm to 15 \u03bcm",
@@ -2980,7 +2980,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "14. The positive electrode active material for a non-aqueous electrolyte secondary battery according to claim 13, wherein the average particle size of the secondary particles is within a range of 1 \u03bcm to 15 \u03bcm, and the value of [(d90\u2212d10)/average particle size], which is an index indicating the spread of the particle size distribution of the secondary particles, is 0.7 or less.",
+        "paragraph": "5. The transition metal composite hydroxide according to claim 1, wherein the average particle size of the plate-shaped primary particles is within a range of 0.3 \u03bcm to 3 \u03bcm, and the average particle size of the fine primary particles is within a range of 0.01 \u03bcm to 0.3 \u03bcm.",
         "measurement_extractions": [
             {
                 "quantity": "0.3 \u03bcm to 3 \u03bcm",
@@ -3001,7 +3001,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "5. The transition metal composite hydroxide according to claim 1, wherein the average particle size of the plate-shaped primary particles is within a range of 0.3 \u03bcm to 3 \u03bcm, and the average particle size of the fine primary particles is within a range of 0.01 \u03bcm to 0.3 \u03bcm.",
+        "paragraph": "6. The transition metal composite hydroxide according to claim 1, wherein the average particle size of the secondary particles is within a range of 1 \u03bcm to 15 \u03bcm to, and the value of [(d90\u2212d10)/average particle size], which is an index that represents the spread of the particle size distribution of the secondary particles, is 0.65 or less.",
         "measurement_extractions": [
             {
                 "quantity": "1 \u03bcm to 15 \u03bcm",
@@ -3022,7 +3022,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "6. The transition metal composite hydroxide according to claim 1, wherein the average particle size of the secondary particles is within a range of 1 \u03bcm to 15 \u03bcm to, and the value of [(d90\u2212d10)/average particle size], which is an index that represents the spread of the particle size distribution of the secondary particles, is 0.65 or less.",
+        "paragraph": "9. A method for manufacturing a transition metal composite hydroxide, wherein the method is for manufacturing a transition metal composite hydroxide which is a precursor of the positive electrode active material for a non-aqueous electrolyte secondary battery by mixing a raw material aqueous solution including at least a transition metal element and an aqueous solution including an ammonium ion donor to form a reaction aqueous solution, and performing a crystallization reaction, the method is characterized in comprising:\na nucleation step in which nucleation is performed in a non-oxidizing atmosphere having an oxygen concentration of 5% by volume or less in which the pH value of the reaction aqueous solution at a standard liquid temperature of 25\u00b0 C. is adjusted to be within a range of 12.0 to 14.0; and\na particle growth step in which at a standard liquid temperature 25\u00b0 C. the pH value of the reaction aqueous solution including the nuclei obtained in the nucleation step is adjusted to be lower than the pH value of the nucleation step and to be within a range of 10.5 to 12.0 so as to grow the nuclei; wherein\nan atmosphere control is performed such that the non-oxidizing atmosphere is maintained in the early period and the middle period of the particle growth step which is in a range of 70% to 90% of time from the initiation of the particle growth step with respect to the entire period of the particle growth step, and in the latter period of the particle growth step, the non-oxidizing atmosphere is switched to the oxidizing atmosphere where the oxygen concentration exceeds 5% by volume, and then the oxidizing atmosphere is switched to the non-oxidizing atmosphere again.",
         "measurement_extractions": [
             {
                 "quantity": "25\u00b0 C",
@@ -3055,7 +3055,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "9. A method for manufacturing a transition metal composite hydroxide, wherein the method is for manufacturing a transition metal composite hydroxide which is a precursor of the positive electrode active material for a non-aqueous electrolyte secondary battery by mixing a raw material aqueous solution including at least a transition metal element and an aqueous solution including an ammonium ion donor to form a reaction aqueous solution, and performing a crystallization reaction, the method is characterized in comprising:\na nucleation step in which nucleation is performed in a non-oxidizing atmosphere having an oxygen concentration of 5% by volume or less in which the pH value of the reaction aqueous solution at a standard liquid temperature of 25\u00b0 C. is adjusted to be within a range of 12.0 to 14.0; and\na particle growth step in which at a standard liquid temperature 25\u00b0 C. the pH value of the reaction aqueous solution including the nuclei obtained in the nucleation step is adjusted to be lower than the pH value of the nucleation step and to be within a range of 10.5 to 12.0 so as to grow the nuclei; wherein\nan atmosphere control is performed such that the non-oxidizing atmosphere is maintained in the early period and the middle period of the particle growth step which is in a range of 70% to 90% of time from the initiation of the particle growth step with respect to the entire period of the particle growth step, and in the latter period of the particle growth step, the non-oxidizing atmosphere is switched to the oxidizing atmosphere where the oxygen concentration exceeds 5% by volume, and then the oxidizing atmosphere is switched to the non-oxidizing atmosphere again.",
+        "paragraph": "1. A carbonate precursor compound for manufacturing a lithium metal (M)-oxide powder usable as an active positive electrode material in lithium-ion batteries, M comprising 20 to 90 mol % Ni, 10 to 70 mol % Mn and 10 to 40 mol % Co, the precursor further comprising a sodium and sulfur impurity, wherein the sodium to sulfur molar ratio (Na/S) is 0.4<Na/S<2, and wherein the sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % is more than 0.4 wt % and less than 1.6 wt %.",
         "measurement_extractions": [
             {
                 "quantity": "is more than 0.4 wt %",
@@ -3070,7 +3070,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "1. A carbonate precursor compound for manufacturing a lithium metal (M)-oxide powder usable as an active positive electrode material in lithium-ion batteries, M comprising 20 to 90 mol % Ni, 10 to 70 mol % Mn and 10 to 40 mol % Co, the precursor further comprising a sodium and sulfur impurity, wherein the sodium to sulfur molar ratio (Na/S) is 0.4<Na/S<2, and wherein the sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % is more than 0.4 wt % and less than 1.6 wt %.",
+        "paragraph": "11. The method according to claim 7, wherein the concentration of NH3in the reactor is less than 5.0 g/L.",
         "measurement_extractions": [
             {
                 "quantity": "less than 5.0 g/L",
@@ -3085,7 +3085,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "11. The method according to claim 7, wherein the concentration of NH3in the reactor is less than 5.0 g/L.",
+        "paragraph": "14. The method according to claim 7, wherein the seeds have a median particle size D50 between 0.1 and 3 \u03bcm.",
         "measurement_extractions": [
             {
                 "quantity": "between 0.1 and 3 \u03bcm",
@@ -3100,7 +3100,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "14. The method according to claim 7, wherein the seeds have a median particle size D50 between 0.1 and 3 \u03bcm.",
+        "paragraph": "15. A method for preparing the carbonate precursor compound of claim 2, comprising:\nproviding a feed solution comprising Ni-, Mn- and Co-ions, and a source of A, wherein the Ni-, Mn-, Co- and A-ions are present in a water soluble sulfate compound,\nproviding an ionic solution comprising a carbonate solution and Na-ions, wherein the CO<sub>3</sub>/SO<sub>4 </sub>rate is selected so as to obtain a Na/S molar ratio with 0.4<Na/S<2 and the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % yield a sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of more than 0.4 wt % and less than 1.6 wt %,\nproviding a slurry comprising seeds comprising M\u2032-ions, wherein M\u2032=NixMnyCozA\u2032n,\nA\u2032 being a dopant, with 0\u2264x\u2032\u22641, 0\u2264y\u2032\u22641, 0\u2264z\u2032\u22641, 0\u2264n\u2032\u22641 and x\u2032+y\u2032+z\u2032+n\u2032=1,\nmixing the feed solution, the ionic solution and the slurry in the reactor, thereby obtaining a reactive liquid mixture,\nprecipitating a carbonate onto the seeds in the reactive liquid mixture, thereby obtaining a reacted liquid mixture and the carbonate precursor, and\nseparating the carbonate precursor from the reacted liquid mixture.",
         "measurement_extractions": [
             {
                 "quantity": "0.4<Na/S<2",
@@ -3121,7 +3121,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "15. A method for preparing the carbonate precursor compound of claim 2, comprising:\nproviding a feed solution comprising Ni-, Mn- and Co-ions, and a source of A, wherein the Ni-, Mn-, Co- and A-ions are present in a water soluble sulfate compound,\nproviding an ionic solution comprising a carbonate solution and Na-ions, wherein the CO<sub>3</sub>/SO<sub>4 </sub>rate is selected so as to obtain a Na/S molar ratio with 0.4<Na/S<2 and the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % yield a sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of more than 0.4 wt % and less than 1.6 wt %,\nproviding a slurry comprising seeds comprising M\u2032-ions, wherein M\u2032=NixMnyCozA\u2032n,\nA\u2032 being a dopant, with 0\u2264x\u2032\u22641, 0\u2264y\u2032\u22641, 0\u2264z\u2032\u22641, 0\u2264n\u2032\u22641 and x\u2032+y\u2032+z\u2032+n\u2032=1,\nmixing the feed solution, the ionic solution and the slurry in the reactor, thereby obtaining a reactive liquid mixture,\nprecipitating a carbonate onto the seeds in the reactive liquid mixture, thereby obtaining a reacted liquid mixture and the carbonate precursor, and\nseparating the carbonate precursor from the reacted liquid mixture.",
+        "paragraph": "5. The carbonate precursor compound of claim 1, wherein the sodium content is between 0.1 and 0.7 wt %, and the sulfur content is between 0.2 and 0.9 wt %.",
         "measurement_extractions": [
             {
                 "quantity": "is between 0.1 and 0.7 wt %",
@@ -3142,7 +3142,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "5. The carbonate precursor compound of claim 1, wherein the sodium content is between 0.1 and 0.7 wt %, and the sulfur content is between 0.2 and 0.9 wt %.",
+        "paragraph": "6. A lithium metal oxide powder for a positive electrode material in a rechargeable battery, having the general formula Li<sub>1+a</sub>M<sub>1\u2212a</sub>O<sub>2 </sub>where M=Ni<sub>x</sub>Mn<sub>y</sub>Co<sub>z</sub>A<sub>v</sub>, A being a dopant, wherein 0.10\u2264a<0.25, 0.10\u2264x<0.30, 0.55\u2264y\u22640.80, and 0<z\u22640.30, v\u22640.05, and x+y+z+v=1, the powder having a particle size distribution with 10 \u03bcm\u2264D50\u226420 \u03bcm, a specific surface with 0.9\u2264BET\u22645, the BET being expressed in m<sup>2</sup>/g, the powder further comprising a sodium and sulfur impurity, wherein the sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % is more than 0.4 wt % and less than 1.6 wt %, and wherein the sodium to sulfur molar ratio (Na/S) is 0.4<Na/S<2.",
         "measurement_extractions": [
             {
                 "quantity": "10 \u03bcm\u2264D50\u226420 \u03bcm",
@@ -3169,7 +3169,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "6. A lithium metal oxide powder for a positive electrode material in a rechargeable battery, having the general formula Li<sub>1+a</sub>M<sub>1\u2212a</sub>O<sub>2 </sub>where M=Ni<sub>x</sub>Mn<sub>y</sub>Co<sub>z</sub>A<sub>v</sub>, A being a dopant, wherein 0.10\u2264a<0.25, 0.10\u2264x<0.30, 0.55\u2264y\u22640.80, and 0<z\u22640.30, v\u22640.05, and x+y+z+v=1, the powder having a particle size distribution with 10 \u03bcm\u2264D50\u226420 \u03bcm, a specific surface with 0.9\u2264BET\u22645, the BET being expressed in m<sup>2</sup>/g, the powder further comprising a sodium and sulfur impurity, wherein the sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % is more than 0.4 wt % and less than 1.6 wt %, and wherein the sodium to sulfur molar ratio (Na/S) is 0.4<Na/S<2.",
+        "paragraph": "7. A method for preparing a carbonate precursor compound according to claim 1, comprising:\nproviding a feed solution comprising Ni-, Mn- and Co-ions, and a source of A, wherein the Ni-, Mn-, Co- and A-ions are present in a water soluble sulfate compound,\nproviding an ionic solution comprising a carbonate solution and Na-ions, wherein the CO<sub>3</sub>/SO<sub>4 </sub>rate is selected so as to obtain a Na/S molar ratio with 0.4<Na/S<2 and the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % yield a sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of more than 0.4 wt % and less than 1.6 wt %,\nproviding a slurry comprising seeds comprising M\u2032-ions, wherein M\u2032=NixMnyCozA\u2032n,\nA\u2032 being a dopant, with 0\u2264x\u2032\u22641, 0\u2264y\u2032\u22641, 0\u2264z\u2032\u22641, 0\u2264n\u2032\u22641 and x\u2032+y\u2032+z\u2032+n\u2032=1,\nmixing the feed solution, the ionic solution and the slurry in the reactor, thereby obtaining a reactive liquid mixture,\nprecipitating a carbonate onto the seeds in the reactive liquid mixture, thereby obtaining a reacted liquid mixture and the carbonate precursor, and\nseparating the carbonate precursor from the reacted liquid mixture.",
         "measurement_extractions": [
             {
                 "quantity": "0.4<Na/S<2",
@@ -3190,7 +3190,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "7. A method for preparing a carbonate precursor compound according to claim 1, comprising:\nproviding a feed solution comprising Ni-, Mn- and Co-ions, and a source of A, wherein the Ni-, Mn-, Co- and A-ions are present in a water soluble sulfate compound,\nproviding an ionic solution comprising a carbonate solution and Na-ions, wherein the CO<sub>3</sub>/SO<sub>4 </sub>rate is selected so as to obtain a Na/S molar ratio with 0.4<Na/S<2 and the sodium (Na<sub>wt</sub>) and sulfur (S<sub>wt</sub>) content expressed in wt % yield a sum (2*Na<sub>wt</sub>)+S<sub>wt </sub>of more than 0.4 wt % and less than 1.6 wt %,\nproviding a slurry comprising seeds comprising M\u2032-ions, wherein M\u2032=NixMnyCozA\u2032n,\nA\u2032 being a dopant, with 0\u2264x\u2032\u22641, 0\u2264y\u2032\u22641, 0\u2264z\u2032\u22641, 0\u2264n\u2032\u22641 and x\u2032+y\u2032+z\u2032+n\u2032=1,\nmixing the feed solution, the ionic solution and the slurry in the reactor, thereby obtaining a reactive liquid mixture,\nprecipitating a carbonate onto the seeds in the reactive liquid mixture, thereby obtaining a reacted liquid mixture and the carbonate precursor, and\nseparating the carbonate precursor from the reacted liquid mixture.",
+        "paragraph": "What is claimed is:\n1. A production method for producing transition metal composite hydroxide particles by a crystallization reaction to be a precursor for a cathode active material for a non-aqueous electrolyte rechargeable battery, comprising:\na nucleation process for performing nucleation by controlling an aqueous solution for nucleation that includes a metal compound that includes at least a transition metal and an ammonium ion donor so that the pH value at a standard liquid temperature of 25\u00b0 C. becomes 12.0 to 14.0; and\na particle growth process for causing nuclei to grow by controlling an aqueous solution for particle growth that includes the nuclei that were obtained in the nucleation process so that the pH value is less than in the nucleation process and is 10.5 to 12.0;\nthe reaction atmosphere in the nucleation process and at the beginning of the particle growth process being a non-oxidizing atmosphere in which an oxygen concentration is 5% by volume or less; and\nin the particle growth process, atmosphere control by which the reaction atmosphere is switched from the non-oxidizing atmosphere to an oxidizing atmosphere in which the oxygen concentration is greater than 5% by volume at timing from the start of the particle growth process within a range of 5% to 35% of the overall particle growth process time, and is then switched from the oxidizing atmosphere to a non-oxidizing atmosphere in which the oxygen concentration is 5% by volume or less so that the crystallization time in the oxidizing atmosphere in the particle growth process is 3% to 20% of the overall particle growth process time being performed at least one time.",
         "measurement_extractions": [
             {
                 "quantity": "12.0 to 14.0",
@@ -3211,7 +3211,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "What is claimed is:\n1. A production method for producing transition metal composite hydroxide particles by a crystallization reaction to be a precursor for a cathode active material for a non-aqueous electrolyte rechargeable battery, comprising:\na nucleation process for performing nucleation by controlling an aqueous solution for nucleation that includes a metal compound that includes at least a transition metal and an ammonium ion donor so that the pH value at a standard liquid temperature of 25\u00b0 C. becomes 12.0 to 14.0; and\na particle growth process for causing nuclei to grow by controlling an aqueous solution for particle growth that includes the nuclei that were obtained in the nucleation process so that the pH value is less than in the nucleation process and is 10.5 to 12.0;\nthe reaction atmosphere in the nucleation process and at the beginning of the particle growth process being a non-oxidizing atmosphere in which an oxygen concentration is 5% by volume or less; and\nin the particle growth process, atmosphere control by which the reaction atmosphere is switched from the non-oxidizing atmosphere to an oxidizing atmosphere in which the oxygen concentration is greater than 5% by volume at timing from the start of the particle growth process within a range of 5% to 35% of the overall particle growth process time, and is then switched from the oxidizing atmosphere to a non-oxidizing atmosphere in which the oxygen concentration is 5% by volume or less so that the crystallization time in the oxidizing atmosphere in the particle growth process is 3% to 20% of the overall particle growth process time being performed at least one time.",
+        "paragraph": "2. A production method for producing transition metal composite hydroxide particles by a crystallization reaction to be a precursor for a cathode active material for a non-aqueous electrolyte rechargeable battery, comprising:\na nucleation process for performing nucleation by controlling an aqueous solution for nucleation that includes a metal compound that includes at least a transition metal and an ammonium ion donor so that the pH value at a standard liquid temperature of 25\u00b0 C. becomes 12.0 to 14.0; and\na particle growth process for causing nuclei to grow by controlling an aqueous solution for particle growth that includes the nuclei that were obtained in the nucleation process so that the pH value is less than in the nucleation process and is 10.5 to 12.0;\nthe reaction atmosphere in the nucleation process and at the beginning of the particle growth process being a non-oxidizing atmosphere in which the oxygen concentration is 5% by volume or less;\nin the particle growth process, atmosphere control by which the reaction atmosphere is switched from the non-oxidizing atmosphere to an oxidizing atmosphere in which the oxygen concentration is greater than 5% by volume, and is then switched from that oxidizing atmosphere to a non-oxidizing atmosphere in which the oxygen concentration is 5% by volume or less being performed two times or more; and\nthe total crystallization reaction time in the oxidizing atmosphere in the particle growth process being 3% to 30% of the total particle growth process time, and the crystallization reaction time during each oxidizing atmosphere being 1% or more of the total particle growth process time.",
         "measurement_extractions": [
             {
                 "quantity": "12.0 to 14.0",
@@ -3232,7 +3232,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "2. A production method for producing transition metal composite hydroxide particles by a crystallization reaction to be a precursor for a cathode active material for a non-aqueous electrolyte rechargeable battery, comprising:\na nucleation process for performing nucleation by controlling an aqueous solution for nucleation that includes a metal compound that includes at least a transition metal and an ammonium ion donor so that the pH value at a standard liquid temperature of 25\u00b0 C. becomes 12.0 to 14.0; and\na particle growth process for causing nuclei to grow by controlling an aqueous solution for particle growth that includes the nuclei that were obtained in the nucleation process so that the pH value is less than in the nucleation process and is 10.5 to 12.0;\nthe reaction atmosphere in the nucleation process and at the beginning of the particle growth process being a non-oxidizing atmosphere in which the oxygen concentration is 5% by volume or less;\nin the particle growth process, atmosphere control by which the reaction atmosphere is switched from the non-oxidizing atmosphere to an oxidizing atmosphere in which the oxygen concentration is greater than 5% by volume, and is then switched from that oxidizing atmosphere to a non-oxidizing atmosphere in which the oxygen concentration is 5% by volume or less being performed two times or more; and\nthe total crystallization reaction time in the oxidizing atmosphere in the particle growth process being 3% to 30% of the total particle growth process time, and the crystallization reaction time during each oxidizing atmosphere being 1% or more of the total particle growth process time.",
+        "paragraph": "6. Transition metal composite hydroxide particles that are the precursor for cathode active material for a non-aqueous electrolyte rechargeable battery, comprising secondary particles that are formed by an aggregation of plate-shaped primary particles and fine primary particles that are smaller than the plate-shaped primary particles;\nthe secondary particles having a center section that is formed by an aggregation of the plate-shaped primary particles, and one layered structure of a low-density section that is formed by an aggregation of the fine primary particles and a high-density section that is formed by an aggregation of the plate-shaped primary particles on the outside of the center section;\nthe average value of the ratio of the center section outer diameter with respect to the particle size of the secondary particles being 30% to 80%, and the average value of the high-density section radial direction thickness with respect to the particle size of the secondary particles being 5% to 25%; and\nthe secondary particles having an average particle size of 1 \u03bcm to 15 \u03bcm, and an index [(d90\u2212d10)/average particle size] that indicates the extent of the particle size distribution of 0.65 or less.",
         "measurement_extractions": [
             {
                 "quantity": "1 \u03bcm to 15 \u03bcm",
@@ -3253,7 +3253,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "6. Transition metal composite hydroxide particles that are the precursor for cathode active material for a non-aqueous electrolyte rechargeable battery, comprising secondary particles that are formed by an aggregation of plate-shaped primary particles and fine primary particles that are smaller than the plate-shaped primary particles;\nthe secondary particles having a center section that is formed by an aggregation of the plate-shaped primary particles, and one layered structure of a low-density section that is formed by an aggregation of the fine primary particles and a high-density section that is formed by an aggregation of the plate-shaped primary particles on the outside of the center section;\nthe average value of the ratio of the center section outer diameter with respect to the particle size of the secondary particles being 30% to 80%, and the average value of the high-density section radial direction thickness with respect to the particle size of the secondary particles being 5% to 25%; and\nthe secondary particles having an average particle size of 1 \u03bcm to 15 \u03bcm, and an index [(d90\u2212d10)/average particle size] that indicates the extent of the particle size distribution of 0.65 or less.",
+        "paragraph": "7. Transition metal composite hydroxide particles that are the precursor for cathode active material for a non-aqueous electrolyte rechargeable battery, comprising secondary particles that are formed by an aggregation of plate-shaped primary particles and fine primary particles that are smaller than the plate-shaped primary particles;\nthe secondary particles having a center section that is formed by an aggregation of plate-shaped primary particles, and two or more layered structure of a low-density section that is formed by an aggregation of the fine primary particles and a high-density section that is formed by an aggregation of the plate-shaped primary particles on the outside of the center section; and\nthe secondary particles having an average particle size of 1 \u03bcm to 15 \u03bcm, and an index [(d90\u2212d10)/average particle size] that indicates the extent of the particle size distribution of 0.65 or less.",
         "measurement_extractions": [
             {
                 "quantity": "1 \u03bcm to 15 \u03bcm",
@@ -3274,7 +3274,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "7. Transition metal composite hydroxide particles that are the precursor for cathode active material for a non-aqueous electrolyte rechargeable battery, comprising secondary particles that are formed by an aggregation of plate-shaped primary particles and fine primary particles that are smaller than the plate-shaped primary particles;\nthe secondary particles having a center section that is formed by an aggregation of plate-shaped primary particles, and two or more layered structure of a low-density section that is formed by an aggregation of the fine primary particles and a high-density section that is formed by an aggregation of the plate-shaped primary particles on the outside of the center section; and\nthe secondary particles having an average particle size of 1 \u03bcm to 15 \u03bcm, and an index [(d90\u2212d10)/average particle size] that indicates the extent of the particle size distribution of 0.65 or less.",
+        "paragraph": "4. The method of claim 1, wherein, when an average particle diameter (D50) of the transition metal precursor is in a range of 5 \u03bcm to 10 \u03bcm, the temperature of the first temperature holding section is in the range of 400\u00b0 C. to 600\u00b0 C.",
         "measurement_extractions": [
             {
                 "quantity": "a range of 5 \u03bcm to 10 \u03bcm",
@@ -3295,7 +3295,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "4. The method of claim 1, wherein, when an average particle diameter (D50) of the transition metal precursor is in a range of 5 \u03bcm to 10 \u03bcm, the temperature of the first temperature holding section is in the range of 400\u00b0 C. to 600\u00b0 C.",
+        "paragraph": "5. The method of claim 1, wherein an average particle diameter (D50) of the transition metal precursor is greater than 10 \u03bcm, the temperature of the first temperature holding section is in the range of 500\u00b0 C. to 650\u00b0 C.",
         "measurement_extractions": [
             {
                 "quantity": "greater than 10 \u03bcm",
@@ -3316,7 +3316,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "5. The method of claim 1, wherein an average particle diameter (D50) of the transition metal precursor is greater than 10 \u03bcm, the temperature of the first temperature holding section is in the range of 500\u00b0 C. to 650\u00b0 C.",
+        "paragraph": "12. Pulverulent compound according to at least one of Claims 1 to 11, characterized in that the normalized width of the particle size distribution, measured according to the Formula (1) D90 -DlO D50 in which D denotes the diameter of the secondary particles, is less than 1.4.",
         "measurement_extractions": [
             {
                 "quantity": "less than 1.4",
@@ -3331,7 +3331,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "12. Pulverulent compound according to at least one of Claims 1 to 11, characterized in that the normalized width of the particle size distribution, measured according to the Formula (1) D90 -DlO D50 in which D denotes the diameter of the secondary particles, is less than 1.4.",
+        "paragraph": "13. Pulverulent compound according to at least one of Claims 1 to 11, characterized in that the normalized width of the particle size distribution, measured according to the Formula (1) D90 -DlO 1) D50 in which D denotes the diameter of the secondary particles, is less than 1.2.",
         "measurement_extractions": [
             {
                 "quantity": "less than 1.2",
@@ -3346,7 +3346,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "13. Pulverulent compound according to at least one of Claims 1 to 11, characterized in that the normalized width of the particle size distribution, measured according to the Formula (1) D90 -DlO 1) D50 in which D denotes the diameter of the secondary particles, is less than 1.2.",
+        "paragraph": "14. Pulverulent compound according to at least one of Claims 1 to 13, characterized in that it has a compressed density of at least 3.2 g/cm3at a compression pressure of 200 MPa.",
         "measurement_extractions": [
             {
                 "quantity": "3.2 g/cm3",
@@ -3361,7 +3361,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "14. Pulverulent compound according to at least one of Claims 1 to 13, characterized in that it has a compressed density of at least 3.2 g/cm3at a compression pressure of 200 MPa.",
+        "paragraph": "15. Pulverulent compound according to at least one of Claims 1 to 14, characterized in that it has a tapped density measured according to ASTM B 527, of at least 2.2 g/cm3.",
         "measurement_extractions": [
             {
                 "quantity": "at least 2.2 g/cm3",
@@ -3376,7 +3376,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "15. Pulverulent compound according to at least one of Claims 1 to 14, characterized in that it has a tapped density measured according to ASTM B 527, of at least 2.2 g/cm3.",
+        "paragraph": "16. Pulverulent compound according to at least one of Claims 1 to 14, characterized in that it has a tapped density measured according to ASTM B 527, of at least 2.4 g/cm3.",
         "measurement_extractions": [
             {
                 "quantity": "at least 2.4 g/cm3",
@@ -3391,7 +3391,7 @@
     },
     {
         "instruction": "\n    You are an expert at extracting quantity, units and their related context from text. \n    Given a paragraph below identify each quantity and its related unit and related context, i.e. the measured entity and measured property if they exist.\n    ",
-        "paragraph": "16. Pulverulent compound according to at least one of Claims 1 to 14, characterized in that it has a tapped density measured according to ASTM B 527, of at least 2.4 g/cm3.",
+        "paragraph": "3. The cathode material of claim 2, having a pressed density equal to or greater than 3.7 g/cm3.",
         "measurement_extractions": [
             {
                 "quantity": "equal to or greater than 3.7 g/cm3",