NiC35N4H26O5(CH2)4(CH)2 is Indium-derived structured and crystallizes in the monoclinic P2_1/c space group. The structure is zero-dimensional and consists of eight 02329_fluka molecules, sixteen 02329_fluka molecules, and four NiC35N4H26O5 clusters. In each NiC35N4H26O5 cluster, Ni(1) is bonded in an octahedral geometry to one N(1), one N(2), one N(3), one O(1), one O(3), and one O(5) atom. The Ni(1)-N(1) bond length is 2.08 Å. The Ni(1)-N(2) bond length is 2.08 Å. The Ni(1)-N(3) bond length is 2.07 Å. The Ni(1)-O(1) bond length is 2.09 Å. The Ni(1)-O(3) bond length is 2.05 Å. The Ni(1)-O(5) bond length is 2.11 Å. There are thirty-five inequivalent C sites. In the first C site, C(28) is bonded in a trigonal planar geometry to one C(25), one C(29), and one C(33) atom. The C(28)-C(25) bond length is 1.47 Å. The C(28)-C(29) bond length is 1.41 Å. The C(28)-C(33) bond length is 1.41 Å. In the second C site, C(29) is bonded in a distorted trigonal planar geometry to one C(28), one C(30), and one H(21) atom. The C(29)-C(30) bond length is 1.39 Å. The C(29)-H(21) bond length is 1.09 Å. In the third C site, C(30) is bonded in a distorted trigonal planar geometry to one C(29), one C(31), and one H(22) atom. The C(30)-C(31) bond length is 1.40 Å. The C(30)-H(22) bond length is 1.09 Å. In the fourth C site, C(31) is bonded in a distorted trigonal planar geometry to one C(30), one C(32), and one N(4) atom. The C(31)-C(32) bond length is 1.41 Å. The C(31)-N(4) bond length is 1.40 Å. In the fifth C site, C(32) is bonded in a distorted trigonal planar geometry to one C(31), one C(33), and one H(23) atom. The C(32)-C(33) bond length is 1.39 Å. The C(32)-H(23) bond length is 1.09 Å. In the sixth C site, C(1) is bonded in a distorted bent 120 degrees geometry to one C(2), one N(1), and one H(1) atom. The C(1)-C(2) bond length is 1.39 Å. The C(1)-N(1) bond length is 1.35 Å. The C(1)-H(1) bond length is 1.09 Å. In the seventh C site, C(33) is bonded in a distorted trigonal planar geometry to one C(28), one C(32), and one H(24) atom. The C(33)-H(24) bond length is 1.09 Å. In the eighth C site, C(34) is bonded in a distorted bent 120 degrees geometry to one O(1) and one O(2) atom. The C(34)-O(1) bond length is 1.28 Å. The C(34)-O(2) bond length is 1.27 Å. In the ninth C site, C(2) is bonded in a distorted trigonal planar geometry to one C(1), one C(3), and one H(2) atom. The C(2)-C(3) bond length is 1.41 Å. The C(2)-H(2) bond length is 1.09 Å. In the tenth C site, C(3) is bonded in a trigonal planar geometry to one C(2), one C(4), and one C(6) atom. The C(3)-C(4) bond length is 1.40 Å. The C(3)-C(6) bond length is 1.47 Å. In the eleventh C site, C(4) is bonded in a distorted single-bond geometry to one C(3) and one H(3) atom. The C(4)-H(3) bond length is 1.09 Å. In the twelfth C site, C(5) is bonded in a distorted bent 120 degrees geometry to one N(1) and one H(4) atom. The C(5)-N(1) bond length is 1.35 Å. The C(5)-H(4) bond length is 1.09 Å. In the thirteenth C site, C(38) is bonded in a distorted bent 120 degrees geometry to one O(3) and one O(4) atom. The C(38)-O(3) bond length is 1.28 Å. The C(38)-O(4) bond length is 1.27 Å. In the fourteenth C site, C(6) is bonded in a trigonal planar geometry to one C(11), one C(3), and one C(7) atom. The C(6)-C(11) bond length is 1.41 Å. The C(6)-C(7) bond length is 1.40 Å. In the fifteenth C site, C(7) is bonded in a distorted single-bond geometry to one C(6) and one H(5,8) atom. The C(7)-H(5,8) bond length is 1.09 Å. In the sixteenth C site, C(8) is bonded in a distorted single-bond geometry to one C(9) and one H(6) atom. The C(8)-C(9) bond length is 1.41 Å. The C(8)-H(6) bond length is 1.09 Å. In the seventeenth C site, C(9) is bonded in a distorted trigonal planar geometry to one C(10), one C(8), and one N(4) atom. The C(9)-C(10) bond length is 1.41 Å. The C(9)-N(4) bond length is 1.40 Å. In the eighteenth C site, C(10) is bonded in a distorted single-bond geometry to one C(9) and one H(7) atom. The C(10)-H(7) bond length is 1.09 Å. In the nineteenth C site, C(11) is bonded in a distorted single-bond geometry to one C(6) and one H(5,8) atom. The C(11)-H(5,8) bond length is 1.09 Å. In the twentieth C site, C(12) is bonded in a distorted bent 120 degrees geometry to one N(2) and one H(9) atom. The C(12)-N(2) bond length is 1.35 Å. The C(12)-H(9) bond length is 1.09 Å. In the twenty-first C site, C(13) is bonded in a distorted single-bond geometry to one C(14) and one H(10) atom. The C(13)-C(14) bond length is 1.40 Å. The C(13)-H(10) bond length is 1.09 Å. In the twenty-second C site, C(14) is bonded in a trigonal planar geometry to one C(13), one C(15), and one C(17) atom. The C(14)-C(15) bond length is 1.40 Å. The C(14)-C(17) bond length is 1.47 Å. In the twenty-third C site, C(15) is bonded in a distorted single-bond geometry to one C(14) and one H(11) atom. The C(15)-H(11) bond length is 1.09 Å. In the twenty-fourth C site, C(16) is bonded in a distorted bent 120 degrees geometry to one N(2) and one H(12) atom. The C(16)-N(2) bond length is 1.35 Å. The C(16)-H(12) bond length is 1.09 Å. In the twenty-fifth C site, C(17) is bonded in a trigonal planar geometry to one C(14), one C(18), and one C(22) atom. The C(17)-C(18) bond length is 1.41 Å. The C(17)-C(22) bond length is 1.40 Å. In the twenty-sixth C site, C(18) is bonded in a distorted single-bond geometry to one C(17), one C(19), and one H(13) atom. The C(18)-C(19) bond length is 1.39 Å. The C(18)-H(13) bond length is 1.09 Å. In the twenty-seventh C site, C(19) is bonded in a distorted trigonal planar geometry to one C(18), one C(20), and one H(14) atom. The C(19)-C(20) bond length is 1.40 Å. The C(19)-H(14) bond length is 1.09 Å. In the twenty-eighth C site, C(20) is bonded in a distorted trigonal planar geometry to one C(19), one C(21), and one N(4) atom. The C(20)-C(21) bond length is 1.40 Å. The C(20)-N(4) bond length is 1.43 Å. In the twenty-ninth C site, C(21) is bonded in a distorted trigonal planar geometry to one C(20), one C(22), and one H(15) atom. The C(21)-C(22) bond length is 1.39 Å. The C(21)-H(15) bond length is 1.09 Å. In the thirtieth C site, C(22) is bonded in a distorted single-bond geometry to one C(17), one C(21), and one H(16) atom. The C(22)-H(16) bond length is 1.09 Å. In the thirty-first C site, C(23) is bonded in a distorted bent 120 degrees geometry to one C(24), one N(3), and one H(17) atom. The C(23)-C(24) bond length is 1.38 Å. The C(23)-N(3) bond length is 1.35 Å. The C(23)-H(17) bond length is 1.09 Å. In the thirty-second C site, C(24) is bonded in a distorted trigonal planar geometry to one C(23), one C(25), and one H(18) atom. The C(24)-C(25) bond length is 1.41 Å. The C(24)-H(18) bond length is 1.09 Å. In the thirty-third C site, C(25) is bonded in a trigonal planar geometry to one C(24), one C(26), and one C(28) atom. The C(25)-C(26) bond length is 1.41 Å. In the thirty-fourth C site, C(26) is bonded in a distorted single-bond geometry to one C(25), one C(27), and one H(19) atom. The C(26)-C(27) bond length is 1.39 Å. The C(26)-H(19) bond length is 1.09 Å. In the thirty-fifth C site, C(27) is bonded in a distorted trigonal planar geometry to one C(26), one N(3), and one H(20) atom. The C(27)-N(3) bond length is 1.35 Å. The C(27)-H(20) bond length is 1.09 Å. There are four inequivalent N sites. In the first N site, N(1) is bonded in a trigonal planar geometry to one Ni(1), one C(1), and one C(5) atom. In the second N site, N(2) is bonded in a trigonal planar geometry to one Ni(1), one C(12), and one C(16) atom. In the third N site, N(3) is bonded in a trigonal planar geometry to one Ni(1), one C(23), and one C(27) atom. In the fourth N site, N(4) is bonded in a trigonal planar geometry to one C(20), one C(31), and one C(9) atom. There are twenty-five inequivalent H sites. In the first H site, H(1) is bonded in a single-bond geometry to one C(1) atom. In the second H site, H(2) is bonded in a single-bond geometry to one C(2) atom. In the third H site, H(35) is bonded in a single-bond geometry to one O(2) and one O(5) atom. The H(35)-O(2) bond length is 1.67 Å. The H(35)-O(5) bond length is 1.01 Å. In the fourth H site, H(3) is bonded in a single-bond geometry to one C(4) atom. In the fifth H site, H(36) is bonded in a distorted single-bond geometry to one O(4) and one O(5) atom. The H(36)-O(4) bond length is 1.67 Å. The H(36)-O(5) bond length is 1.01 Å. In the sixth H site, H(4) is bonded in a single-bond geometry to one C(5) atom. In the seventh H site, H(5,8) is bonded in a single-bond geometry to one C(7) atom. In the eighth H site, H(6) is bonded in a single-bond geometry to one C(8) atom. In the ninth H site, H(7) is bonded in a single-bond geometry to one C(10) atom. In the tenth H site, H(9) is bonded in a single-bond geometry to one C(12) atom. In the eleventh H site, H(10) is bonded in a single-bond geometry to one C(13) atom. In the twelfth H site, H(11) is bonded in a single-bond geometry to one C(15) atom. In the thirteenth H site, H(12) is bonded in a single-bond geometry to one C(16) atom. In the fourteenth H site, H(13) is bonded in a single-bond geometry to one C(18) atom. In the fifteenth H site, H(14) is bonded in a single-bond geometry to one C(19) atom. In the sixteenth H site, H(15) is bonded in a single-bond geometry to one C(21) atom. In the seventeenth H site, H(16) is bonded in a single-bond geometry to one C(22) atom. In the eighteenth H site, H(17) is bonded in a single-bond geometry to one C(23) atom. In the nineteenth H site, H(18) is bonded in a single-bond geometry to one C(24) atom. In the twentieth H site, H(19) is bonded in a single-bond geometry to one C(26) atom. In the twenty-first H site, H(20) is bonded in a single-bond geometry to one C(27) atom. In the twenty-second H site, H(21) is bonded in a single-bond geometry to one C(29) atom. In the twenty-third H site, H(22) is bonded in a single-bond geometry to one C(30) atom. In the twenty-fourth H site, H(23) is bonded in a single-bond geometry to one C(32) atom. In the twenty-fifth H site, H(24) is bonded in a single-bond geometry to one C(33) atom. There are five inequivalent O sites. In the first O site, O(1) is bonded in a bent 120 degrees geometry to one Ni(1) and one C(34) atom. In the second O site, O(2) is bonded in a distorted water-like geometry to one C(34) and one H(35) atom. In the third O site, O(3) is bonded in a distorted bent 120 degrees geometry to one Ni(1) and one C(38) atom. In the fourth O site, O(4) is bonded in a distorted water-like geometry to one C(38) and one H(36) atom. In the fifth O site, O(5) is bonded in a distorted water-like geometry to one Ni(1), one H(35), and one H(36) atom. Linkers: 1 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,1 [CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH].[CH][N].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C].[C]C=[CH].[C][CH].[C][CH].[C][CH].[C][C].[C][C].[C][C].[C][C].[C][C].[C][C]/[C]=[C]/[C]=C(\[C])[N].[C][C]=[CH].[C][N].[C][N].[C][N].[C][N][C].[C][N][C].[C][N][C].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[H].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[N].[Ni].[Ni].[O].[O].[O].[O].[O].[O][Ni] ,2 [O]C(=O)[C@H]1CC[C@H](C([O])=O)CC1. Metal clusters: 2 O.O=[C]O[Ni]O[C]=O. The MOF has largest included sphere 4.33 A, density 1.19 g/cm3, surface area 5068.55 m2/g, accessible volume 0.30 cm3/g