Unrecognizable languages relationship to NP-hard languages
There are NP-hard languages arbitrarily high in the arithmetical hierarchy.

To answer your specific question, the complement of the halting problem is NP-hard and it's in $\mathrm{coRE}\setminus\mathrm{R}$. To see this, let $M$ be a Turing machine that tries all variable assignments for a $\mathrm{SAT}$ instance.  Let it loop forever if it finds a satisfying assignment and let it halt if it doesn't, or if the input isn't a valid encoding of a $\mathrm{SAT}$ instance.  Now, for any string&nbsp;$x$, $x\in\mathrm{SAT}$ iff $\langle M\rangle,x\in\overline{\mathrm{HALT}}$ so we have a reduction from $\mathrm{SAT}$ to the complement of the halting problem.