Switch chrome interface from smartphone mode to tablet mode
You will need to change the DPI of your phone to accomplish it. But, the change will affect the whole system not just Chrome and may not be retained after a restart due to your device not been rooted.

adb shell wm density 600 (When I tested, 600 was the value that enabled the change of interface in Chrome).

For those who have newer version of Android, the DPI can be changed by going to Settings -> System -> Developer Option -> Smallest width.

Chrome's interface will change from phone to tablet.