HD44780 Extended non-display DDRAM?
I haven't used that particular library but I have used the ddram and cgram as memory / buffets. So the feasibility is never in question.

The downside with this approach is speed and real estate. Those devices are slow by mcu standard. You then have to provision for the rw pin and the data pins - both read and writes. That's what you should check for in the library.

But it is workable for sure.