as they were described, allowed the first Raman absorption spectroscopy measurements to be made. In 1970 Alfano and Shapiro reported the first measurements of frequency broadening in crystals and glasses using a frequency doubled Nd:Glass mode-locked laser. The output pulses were approximately 4 ps and had a pulse energy of 5 mJ. The filaments formed produced the first white light spectra in the range from 400-700 nm and the authors explained their formation through self-phase modulation and four-wave mixing. The filaments themselves were of no real use as a source; nevertheless the authors suggested that the crystals might prove useful as ultrafast light gates. Alfano is the discoverer and inventor of the supercontinuum in 1970 with three seminal articles in same issue of Phy Rev Letters (24, 592,584,1217(1970)) on ultimate white light source now called supercontinuum. The study of atomic vapours, organic vapours and liquids by Raman absorption spectroscopy through the 1960s and 1970s drove the development of continua sources. By the early 1970s, continua formed by nanosecond duration flash lamps and laser-triggered breakdown spark in gases, along with laser excited fluorescence continua from scintillator dyes, were being used to study the excited states. These sources all had problems; what was required was a source that produced broad continua at high power levels with a reasonable efficiency. In 1976 Lin and Stolen reported a new nanosecond source that produced continua with a bandwidth of 110-180 nm centred on 530 nm at output powers of around a kW. The system used a 10-20 kW dye laser producing 10 ns pulses with 15-20 nm of bandwidth to pump a 19.5 m long, 7 μm core diameter silica fibre . They could only manage a coupling efficiency in the region of 5-10%. By 1978 Lin and Nguyen reported several continua, most notably one stretching from 0.7-1.6 μm using a 315 m long GeO doped silica fibre with a 33 μm core. The optical setup was similar to Lin's previous work with Stolen, except in this instance the pump source was a 150 kW, 20 ns, Q-switched Nd:YAG laser. Indeed, they had so much power available to them that two thirds was attenuated away to prevent damage to the fibre. The 50 kW coupled into the fibre emerged as a 12 kW continuum . Stokes lines were clearly visible up to 1.3 μm, at which point the continuum began to smooth out, except for