Radin's first EP and the song "Winter" from Radin's record We Were Here. In 2007, Cary Brothers signed a record deal with indie label Bluhammock Music for the release of his first full-length album, Who You Are, on May 29, 2007, which made the Billboard Heatseekers Chart. Produced by Chad Fischer (Alexi Murdoch) and mixed by Greg Collins (Grammy Winner – U2), the record features guest musicians Matt Hales from Aqualung and Priscilla Ahn. The video for the single "Ride" starring Brittany Snow was added to the rotation on VH1 in the U.S. In addition, the record won "Best Rock Album of 2007" by the Indie Acoustic Project. Brothers' track 'Ride' has also been mixed by Tiësto and was a success on the dancefloors of Europe in 2008. He helped close Friday night at Bonnaroo in the summer of 2008 by making a guest appearance with Tiësto and repeated this musical pairing a few months later at the O2 arena in London. In 2009, Brothers went into the studio to work on his second full-length record. In addition, that year he had an original track called "Here on Earth" on the Tiësto record Kaleidescope alongside Sigur Rós, Tegan and Sara, Kele Okereke, Priscilla Ahn and Emily Haines. Under Control was released on April 6, 2010, through Brothers' own Procrastination Music label and premiered at No. 1 on the iTunes Singer-Songwriter charts and No. 10 on the Billboard Heatseekers Chart. Cary toured extensively in the United States in support of the record in 2010 and 2011 as both headliner and as an opening act for the Sara Bareilles tour. Staying active in social media, Brothers was named No. 14 on Paste Magazine's "50 Musicians Worth Following on Twitter" in August 2011. In May 2012, Brothers released a DIY collection of five cover songs entitled Covers Volume One, featuring songs by Yeah Yeah Yeahs, David Bowie, Duran Duran, INXS, and Matt & Kim. The EP also features guest vocals by Rachael Yamagata, Butterfly Boucher, and Priscilla Ahn. It premiered in the Top Ten on the iTunes Singer-Songwriter Chart. In addition, Brothers released the EPs "Let Me Be" in 2014 and "Lovin' On You" in 2015. After touring the US and Europe in 2015 and 2017, Brothers third full-length record "Bruises" was released on April 27, 2018. The single “Crush" went Top 5 on KCRW's influential Morning Becomes Eclectic radio show. Personal life