(voiced by Paul Winchell) - An artist who brings to life anything that he paints. Televisitron (voiced by Hal Smith) - A villain who uses a remote control to send his foes into various channels of the television to do them in. The Impossibles steal Televistatron's remote and transport him into a prison show. Aquator (voiced by Paul Winchell) - An aquatic villain who steals a formula for changing the size of organisms in an attempt to create an army of giant-sized micro-organisms. Dragster (voiced by Paul Winchell impersonating Boris Karloff) - A speedy car thief with who steals a diamond-encrusted car. Puzzler (voiced by Paul Frees) - A supervillain who can change shape as a living puzzle. He is the only villain given an origin as he mentions to have fallen into a jigsaw-making machine which gave him his abilities. Surfer (voiced by Don Messick) - A villain who surfs and uses a remote-control ukulele. Sculptor (voiced by Lennie Weinrib) - A villain who carries a gun that fires quick-dry cement either turning people into statues or making instant rocks and walls. Spraysol (voiced by Hal Smith) - A villain who sports a helmet that sprays liquid or gas. He also speaks with a lisp. Diamond Dazzler (voiced by Alan Reed) - A villain who steals a diamond that contains a genie (voiced by Hal Smith). He carries multiple magic gemstone rings with different abilities. Twister (voiced by Don Messick) - A villain who dresses like a top with a propeller beanie who steals by spinning like a twister. Cronella Critch (voiced by Janet Waldo) - A witch who robbed a charity-for-orphans party. She was turned into a cat due to a spell reversal by Multi-Man. Tapper (voiced by Hal Smith) - A villain who can travel through telephone wires with his weapon, the Deciminator, which he uses to send Coil Man to Ackbar the Martian (voiced by Don Messick) in his flying saucer and Multi Man to Captain Cutlass (voiced by Alan Reed) on his smuggling ship the Sea Serpent. Angler (voiced by [Don Messick) - A villain who wears a torpedo-shaped fish suit that steals with a fishing rod. Ringmaster (voiced by Hal Smith) - A ringmaster-themed villain who has circus performers as his henchmen. Mr. Instant (voiced by Paul Frees) - A villain who carries a gun that can create anything in an instant. Dr. Futuro