The main paragraph text follows directly on here. Interfaces (gas-liquid, gas-solid and liquid-solid) are ubiquitous in nature (aerosol, mist, cell membrane, etc.) and technology (on-water chemistry, electrical double layer, microdroplets, etc.). Among them, gas-liquid interfaces have drawn extensive interests in scientific and engineering community because many fantastic phenomena and processes have been associated with specifically different properties of the interfaces from single phases, i.e., dramatical acceleration of many chemical and photochemical reactions, implying potential applications in atmospheric, biological, biomedical, prebiotic, electrochemical, geochemical, photochemical and synthetic chemistry. Despite substantial progress over the past decades, current investigations of gas-liquid interface are limited to aqueous interface, where gas-organic interface remains neglected and our understanding to the fundamental mechanisms and general uses is hence impaired.