Nevertheless, it is evident that more synergistic efforts, combining the strengths of both high-pressure experiments and computations, are needed. In such studies, experiments will need to deliver high-quality benchmark data for the applied simulation methods, allowing to test their reliability in reproducing experimental observations and to optimize the computational protocols in return. Dedicated model experiments, as described in Section 2.1.2, will play an important role in this regard. Due to the level of sophistication and the complexity of the experimental setups, it is likely that extensive developmental work in the realm of computational high-pressure chemistry will be carried out throughout the coming decades.