To advance the MAPs and overcome existing constrains , we introduce the AUTO-MISCHBARES, a reliable opensource framework designed for fully unsupervised operations. Building upon our earlier work in multithreaded asynchronous web-based frameworks , it integrates real-time analysis and feedback, thus enhancing experimental processes. This platform, features automated capabilities for a range of electrochemical measurements, as showcased in our study of the CEI on battery electrodes. We conducted sequential measurements by utilizing an open-cell setup and characterized them using near-ambient pressure X-ray photoelectron spectroscopy (XPS). The agnostic nature of our framework ensures its adaptability for diverse organic and inorganic materials. This platform not only can accelerate research but also facilitates the sharing of validated data, helping scientist in the efficient extraction and transfer of information within the community .