Future work to improve the accuracy of the parameterisation includes mapping the lithium concentration of the thermal parameters (e.g. specific heat capacity and thermal conductivity), rather than at a single stoichiometry. This relationship was not considered here due to the stability of active materials in ambient conditions. In situ methods that allow measurement as a function of lithium concentration would allow the changes in these parameters that occur during battery operation to be captured. Additionally, the requirement to increase the solid-phase diffusivity value of each electrode highlights limitations in the analytical approach and DFN theory. It is assumed that particles are spherical and monodisperse despite the electrode microstructure being heterogeneous. Ignoring these effects in parameter evaluation and the model is one of the main reasons for disagreement with experimental data. Accounting for electrode inhomogeneity will improve model accuracy, for example including size distribution and non-spherical morphologies.