Finally, the applicability of the used DFT-MD + 2PT methodology is not limited to metal-water interfaces only. Some applications relevant to electrocatalysis, electrochemistry, and materials science include the study of pH and electrolyte effects on the interfacial liquid thermodynamics and structure. While studying such systems might necessitate longer simulation timescales or the use of more sophisticated functionals, the computational approach itself is very general and reasonably efficient for large-scale DFT-MD studies.