The literature has revealed that non-conventional solvents, such as ionic liquids (ILs) and DES, display intricate structures influenced by composition. Microheterogeneities, observed within these systems, including ChCl-carboxylic acid systems , are closely tied to their potential applications . Particularly, the microheterogeneous structure of ChClbased DES materials has been shown to vary with factors such as the cation's alkyl chain length, the HBD ratio, and water content.