We investigated the effect of NIR light actuation on three bimorph actuators: TMC, TMC-CNF, and plasma-ALE treated TMC-CNF (TMC-CNF-Plasma), with a relative humidity of 33%. Figures them, TMC-CNF-Plasma showed the greatest degree of bending, forming a U-shape. For quantitative comparison, the bending angle versus time was measured (see Figure ). The maximum bending angle for TMC is 65°, which rises to 127° with the addition of CNFs. Ultimately, the TMC-CNF-Plasma actuator achieves the highest maximum bending angle of 165°. These results demonstrate that plasma-enabled ALE treatment significantly enhances the light-driven actuating performance of TMC/CNF under NIR exposure.