As this study is a first foray in DSL synthesis for quantum chemistry simulations, we identified several limitations of our approach. Here, we discuss the most important ones. A full overview is provided in the Supplementary Materials. First, we did not test the performance of all the implemented prompt engineering techniques on finetuned models. Given the low impact of prompt engineering beyond the 'Basic' approach on the base model, we suspect that performance differences would likely be more pronounced on finetuned models. Hence, followup work should investigate the impact of different prompt engineering approaches more comprehensively. Nevertheless, we do not expect substantial performance improvements from alternative prompt engineering techniques.