To generate microstructures, the LC E7 mixture employed in the previous sec�on was replaced with a printable LC ink that can be photopolymerized via 2PLP. This ink was adapted from our previous work and consisted of a mixture of LC monomer (C6BP, 29.4 wt%), crosslinkers (RM257 and C6BAPE, 14.7 wt% each), a photoini�ator (BAPO, 1.5 wt%), and an inhibitor (BHT, 0.5 wt%) to prevent thermal polymeriza�on during the alignment process (See Sec�on S4 in the Suppor�ng Informa�on).