In Algorithm 5, we present the pseudocode for the update of t abcd ijkl amplitudes with off-diagonal LMO Fock matrix elements. In a similar procedure as iterative DLPNO-CCSD(T), the energy contribution for off-diagonal LMO Fock matrix elements is computed iteratively (Equations 23 and 24). Unlike the (Q0) algorithm, the iterative (Q) algorithm requires the storage of t abcd ijkl and Γ abcd ijkl for every quadruplet ijkl. The memory costs remain linear-scaling in the limit of larger systems, but can still be significant for the systems studied in this work if the the tighter QNO tolerances are used. To ensure that the memory costs do not grow out of proportion, we define strong and weak quadruplets by sorting each non-screened quadruplet by its energy contribution after a DLPNO-(Q0) computation. The leading quadruplets whose energy contributions add up to at least 90% of the total (Q0) energy are deemed "strong quadruplets" and the rest "weak quadruplets". This procedure is inspired by the procedure used in DLPNO-CCSD(T1). The QNOs, Γ abcd ijkl , and semicanonical t abcd ijkl amplitudes are computed for strong quadruplets at T CUT QNO × T STRONG SCALE QUADS , and weak quadruplets at T CUT QNO × T WEAK SCALE QUADS .