As there are 6 possible FF combinations, this results in 18 isotherms for both CO2 and N2 using 378 unique adsorption points. In total, 24,840 isotherms are generated across 690 MOFs which span different pressures, temperatures, charge assignment methods, and generic forcefield parameters. We refer to the data generated using this subset of MOFs as the Charge-dependent, Reproducible, Accessible, Forcefield-dependent, and Temperaturedependent Exploratory Database of isotherms, or CRAFTED isotherms for brevity. To provide an initial seed for future benchmarking efforts, we make the CRAFTED database (v1.1.1) and scripts available to the broader scientific community in a dedicated Zenodo repository at . This data was obtained using a HTCS workflow that has been developed 56 and validated elsewhere. For more technical details on the GCMC simulations, see the supporting information (SI), supplementary note 1.