The average binding free energies show that the SA-DMA clusters more rapidly reach an almost constant value compared to the SA-AM system. In addition, it is clear that the average binding free energy does not entirely level out but continues to slightly stabilize the cluster as it grows. We speculate that the average binding free energy reaching an almost constant value indicates that we are transitioning from discrete cluster configurations toward a dynamic continuum of cluster states. This hypothesis is backed by the encapsulation of ammonium/dimethylaminium ions, which begin to resemble a solution. For SA-AM, this occurs around 8-10 acid-base pairs, whereas for SA-DMA, it occurs already around 5-6 acid-base pairs.