The two different radii of curvature in a pendent drop leads to the anisotropic stresses due to the interfacial deformation (Kotula and Anna 2016). Compression of aged asphaltenescovered water droplet in a region of low interfacial viscosity could result in no distortion is visible on the droplet while the interfacial tension is still reducing or result in wrinkles appearing on the droplet to relax the large compressional stresses . However, the droplet will return to the laplacian shape over stopping the compressional mode and compressional modulus decreases to reach the plateau ). This observation is in contrast with gel point rheology, where decreasing the modulus by increasing the concentration is unexpected . At high elasticity, strong birefringence is observed upon contracting the aged oil droplet containing asphaltenes using cross-polarized light microscopy which is an indication of particles ordering within the interface . It is also reported that at high concentration, the skin remains on the droplet even after the re-expansion .