x,S1 is the LR-TDHF S 1 state dipole moment and µ RT x,avg is the average RT-TDHF dipole moment (see Figure ). We find that System 1 completes ∼48% of the charge transfer when starting at -1.12 D and ending at an average value of ∼-1.97 D. The RT-TDHF dipole moment for System 2 also approaches the LR-TDHF S 1 dipole moment, but again falls short, obtaining an average value of ∼-3.44 D and completing only ∼64% of the expected charge transfer. Additionally, System 2 shows significant dipole oscillations that are larger in magnitude than the total change in dipole moment from the ground state. Similarly, System 3 does not quite get to the LR-TDHF S 1 dipole moment, but the average dipole moment of ∼-4.57 D yields ∼69% of the charge transfer, so completes the most of all three molecules. Similar to System 2, the dipole oscillations of System 3 are very large. These large dipole oscillations suggest a mixed state for RT-TDHF, whereas nearly identical MO occupations with TDCIS produce very little dipole oscillations, suggesting a near-stationary state.