For the bond-angle parameter scan we ran folding simulations for 31 sets of θ B from θ B = 100 • to θ B = 160 • in increments of 2 • . Figure shows radar plots of a subset of this parameter scan, with foldamer structures and metrics being shown for increments of 4 • . We show structures and metrics up to θ B = 144 • , as all structures beyond this point have similar structures to the minimum energy cluster for θ B = 144 • . All summary metrics for the entire parameter scan are shown in section S6 and all energy vs cluster RMSD plots for the structures shown in this parameter scan are shown in section S9. We note for some examples in the θ B parameter scans we identified cases where sampling of the minimum energy clusters did not adequately capture both left-and right-handed versions the folded structures. We present energy vs. cluster RMSD plots for all structures presented in the two parameter scans in section S8 and section S9. One instance of poor sampling was identified where only a single helical minimum energy cluster was identified.