One might be tempted to use the common goodness-of-fit metric ! " to describe the consistency of the overpolarization predictions, but it is important to note that the correlation -or strength of linear relationship -between the response variable (the calculated dipole moments, # $%&$ ) and explanatory variable (the experimental dipole moments, # '()* ) is very strong regardless of the electronic structure method employed. Therefore, such a metric is unlikely to reveal meaningful differences between various electronic structure methods. To examine the consistency of the predicted overpolarization of each method, we instead elected to perform an analysis of the residuals arising from each linear regression model. Methods that yield more consistent overpolarization should yield residuals that are on average smaller than methods for which strength of the overpolarization varies considerably.