To demonstrate this ability, the OpenFF 1.0.0 (openff-1.0.0), GAFF 1.8 (gaff-1) and GAFF 2.1 (gaff-2) force fields were assessed against a data set of 103 density ( ), 101 enthalpy of mixing Δ ( ) and 100 excess molar volume ( ) data points measured at ambient conditions for a set of binary systems each at three different compositions (25%, 50% and 75%). It contains a total of 36 unique binary mixtures of 39 unique components, and all data points were sourced directly from the ThermoML archive using the framework's built in parsers. All calculation were performed using v0.3.1 of the framework and using the default calculation schemas as described in the documentation .