Numerous electronic elements, including thermoelectric power generators, sensors, energy storage units, antennas, and light-emitting devices, have been successfully embedded into fabrics to serve functions such as monitoring, security, motion sensing, health tracking, and radio-frequency communication. Inkjet printing stands at the forefront of printed electronics technology. The primary benefits of this technology encompass digital and additive patterning, minimizing material wastage, and its adaptability to a wide range of substrates featuring varying levels of mechanical flexibility and form factors. However, the major challenge with printing low-viscosity inkjet inks onto a coarse and permeable textile surface arises due to the ever-shifting arrangement of fibres or yarns and the continuous alteration of fibre structure caused by the interaction of water molecules with the environment. To address the challenges, an interface paste (DM-INS-2510) was applied via screen printing as surface pretreatment on the rough and porous textile substrate before inkjet printing of the MOF ink.