The primary hydrogel network composed of polyacrylamide (PAM). Although PAM hydrogels are commonly used and easily tunable, the low viscosity of the hydrogel precursor may be a reason it is only infrequently used for extrusion printing. The addition of PEDOT:PSS, as shown in this work, dramatically increases the ink viscosity and provides improved characteristics for extrusion printing. The addition of GOPS crosslinks PSS chains, creating a polymer double-network within the hydrogel, insuring that PEDOT:PSS does not diffuse out of the gel or lose its structure. When preparing the inks, PEDOT:PSS, AM, GOPS, and BIS were added to deionized water first, mixed and sonicated for one minute. The solution was then stirred continuously for 1.5-2 hours to allow the PEDOT:PSS to become homogenously mixed. Then the LAP photoinitiator stock solution was added while stirring. The MC was added last and, due to the resulting viscosity, needed to be mixed with a spatula. Each of these inks contained 1.4 g AM and 0. Based on the exploration of parameters above, we chose to maximize flexibility and conductivity for the ink used in the diodes and strain stiffening device. To do so, we used the lowest quantity of MC and BIS (8 wt% and 0.1 wt% respectively) and the highest quantity of PEDOT:PSS (2 wt%) within the range tested. All other components remained the same as the reference ink.