The second aspect tackled is the overpolarization of Cl , which is corrected by applying the Tang Toennis damping function. Only minor modifications are observed in the 1:1 ratio, mainly in the Cl -LAOH interaction, pointing out to the fact that this is the interaction that depends most on the charge-induced dipole interactions of the system. The description of the Cl -Cl RDF, is also improved by the overpolarization correction (see Figure ) as compared to the AIMD calculations, but only in terms of the g(r) value. The position of the first peak does not shift across the three employed force fields, which stays with a deviation of 100 pm from the AIMD spectra. The Tang Toennis correction did induce a shift of 200 pm the Cl -Cl peak of the ChCl-EG system, leading to a disagreement of 70 pm with AIMD, not far from the di↵erence in our system for all the force field versions. However, the Cl anions were predicted to be further away from each other by AIMD calculation in that system, pointing out to a less structured environment with significant influence of the polarization e↵ects. We can conclude that the Tang Toennis correction does not cruciallly alter the structure of the system at this point. This already suggests the lack of relevance of the Cl -LAOH interaction in the system, the most susceptible interaction among the three charge-dipole interactions. This is probably due to the fact that the main interaction between ChCl and LA is the one taking place with the carboxylic moiety, on the contrary to other systems in the literature having solely an alcohol group in the neutral molecule.