Building on our benchmark calculations, we calculated the harmonic IR and Raman spectra of acetone in three different solvents. We used the PBE0/pcseg-2 level of theory with a polarizable solvent sphere of 16 Å radius and a non-polarizable outer sphere of 30 Å radius. Approximately 250 snapshots were used with a step size of 2.0 ps between them. The eight lowest-frequency modes were removed based on the pseudo-translational and pseudo-rotational analysis. We compared the solvent shifts of the carbonyl stretching mode to the experimental ones, revealing errors ranging from 9-23 cm -1 . Additionally, we compared our simulated Raman spectrum for acetone in water to an experimental spectrum, displaying many similarities between the spectra. The largest frequency deviations, about 25 cm -1 , were observed between 1000-1500 cm -1 .. The largest deviations in Raman intensities were observed for the C-C stretching mode at around 830 cm -1 and the carbonyl stretching mode at around 1769 cm -1 .