The enhancement of plasma-ALE treatment on vacuum-filtered actuators has been previously mentioned, with the maximum bending angle increasing from 127° to 165° (see Figure ). Leveraging the highresolution capabilities of AJP, we designed three-strip patterns for the printed actuator, with each strip approximately 3 mm wide. Upon NIR light illumination, the printed actuator exhibited pronounced arched deformation, with the middle part contracting the most and achieving the largest bending angle of 21° (Movie S4). This angle doubled after plasma-ALE treatment (Movie S5), attributed to the change from Fdominated to O-dominated surface terminations and significantly enhanced light-driven performance.