Disordered structures differ from ordered ones in that they intrinsically exhibit a broad distribution of particle-level resonant frequencies, reflecting how particles' diverse local environments can impact their interactions with light. Changes to microstructure that increase the variance of single-particle resonant frequencies also lead to linewidth broadening in the far-field. For all macrostates examined, we find that there is a strong negative correlation between a particle's resonant frequency and its near-field enhancement, quantified by the maximum electric field intensity on the particle's surface (i.e., particles with redshifted resonant frequencies have more intense surface hotspots). Moreover, nanoparticles with similar resonant frequencies form anisotropic and oriented structures, despite being embedded within an isotropic and disordered microstructure. These collectively resonating clusters can be tuned with the frequency and polarization of incident light. These observations suggest new avenues for using controlled assembly of disordered colloidal macrostates to create materials with distinctive optical properties. They also suggest novel ways light may be used to dynamically manipulate the structure and properties of disordered plasmonic assemblies.