Overall, driving the RT-TDHF MO occupation to what would be expected for the S 1 state produces an electron density indicative of some charge transfer, but not as much as would be expected from the LR-TDHF S 1 dipole moments. In all cases, the RT-TDHF average dipole moment is smaller than the corresponding LR-TDHF value, showing that the charge transfer is incomplete. There is a size-dependent trend in the degree of charge transfer, with System 1 showing the largest disagreement in the dipole moment charge compared to linear response theory, with some improvement with increasing system size. However, the improvement in the average dipole moment change for Systems 2 and 3 comes with a large dipole oscillation, supporting that the systems are in a mixed state. A mixed state at equal population of the HOMO and LUMO agrees with the finding in some previous work by one of the authors that suggests that single electron occupation of the HOMO and LUMO with single determinant RT-TDHF may be more representative of a mixed state composed half of the S 0 state and half of the doubly excited S 2 state, rather than the S 1 state.