Similarly as in Section 6.2, we compare the computed static and MD-based Raman spectra to experiment. The Raman spectra for the dry COF-1 are presented in Figure . The intensities of the static Raman spectrum were computed from DFPT polarizabilities. In the MD case, we employ three different methods. These methods include the polarizability tensors calculated from induced dipole moments (Equation ( )), denoted as α (µ ind ), and the DFPT approach (Equation ( )), denoted as α DFPT . We computed the induced dipole moments using the Berry phase scheme and MLWFs.