In conclusion, we report scalable quasiperiodic patterns in isoreticular Moiré metal-organic frameworks (MOFs). Compared to conventional quasicrystals, MOFs offer the advantage of tunable structures, enabling systematic modulation of the length scale in Zr-NDC, Zr-BPDC, and Zr-AZDC, with edge lengths of 6.13, 6.85, and 7.57 nm, respectively, corresponding to the size of the Stampfli tiles at the 3 rd inflation. By employing mathematical derivation, we demonstrated that these patterns are indeed aperiodic, paving the way for investigating sizedependent properties and uncovering novel physical behaviors. This study provides valuable insights into the formation of quasiperiodic patterns within highly ordered MOFs. The structural diversity of MOFs further creates opportunities to explore various quasiperiodic arrangements, including octagonal quasiperiodic pattern (Figure ). We anticipate the development of synthetic strategies for the intentional design of specific angles in twisted bilayer MOFs, which hold the potential of twistronics to precisely control electrical, magnetic, and optical properties.