A limited number of simulation and experimental studies investigating the surface morphology of matrix-isolated N2 have been performed. Experimental characterization studies of the crystal structure of N2 indicate that there are three structural forms: α-N2, β-N2, or γ-N2. While the temperatures and pressures needed to form γ-N2 are outside of the range of this experiment, both α-N2 and β-N2 packing motifs are possible when depositing a room-temperature gas phase mixture onto a 10 K substrate. As shown experimentally by Beker et al., through X-ray diffraction and IR spectroscopy, molecular N2 deposited under matrix-isolation conditions forms a particularly porous surface due to the random orientation of N2 molecules on the cold substrate. As a result, incoming molecules used in the study (Ar and CH4) were trapped easily in the large pores in the N2 layer. It has been noted, however, that high-level modeling specifically of the deposition process of matrix-isolated N2 is currently unattainable based on inadequate documentation of the needed pair potential. Based on the limited literature available, we predict that the surface roughness of N2 increases with larger deposition angles. This increased surface roughness exhibits an increase in surface deformities and pockets for CH3ONO trapping.