, where the local excitation on chromophore is coupled to solvent→chromophore charge-transfer excitations; (v) full ALMO-TDA+CT, where all the possible local and chargetransfer excitations are incorporated. From a bottom-up view, the contrast between (iii) and (i) should be able to indicate the changes in excitation energies due to the entanglement of virtual orbitals (V C and V S ), while the contrast between (iv) and (i) should correspond to the effect of occupied orbital entanglement (O C and O S ).