In contrast to previous work, the pair selection thresholds are no longer used to categorize orbital pairs into sets with different accuracy settings (TIGHTPNO, NORMALPNO, or LOOSEPNO) but rather to separately control single DLPNO thresholds while aiming at a target accuracy of either TIGHTPNO or NORMALPNO. This allows for an independent control over the domain approximation and pair approximation through τ ∆ CutPNO and τ ∆ CutPairs , respectively. Additionally, for reducing the number of orbital pairs in the CCSD residual equations compared to previous work, we propose to release the constraint for the threshold τ CutPairs of an orbital pair i j to evaluate to the minimum value of τ CutPairs found for any orbital pair that includes i or j. This constraint was originally introduced in Ref. 26 to avoid unstable amplitude optimizations. Therefore, τ ∆ CutPairs influences the stability of the CCSD amplitude optimizations and has to be chosen carefully.