Many different types of materials form sheaf-like and spherulite superstructures. Examples of hyperbranched crystalline natural materials are minerals including stilbite, calcium oxalate, uric acid, fluorapatite. Such morphologies have also been observed in inorganic salts: Bi2S3, 4 metal phosphides, BaSO4, and LnVO4, 8 just to name of few. Polymers including proteins and metals are known to appear also as spherulites. The properties of crystalline materials have been shown to be strongly dependent on their morphologies. For example, mesoporous sheaf-like cobalt oxide functions as superior anode for rechargeable lithium-ion batteries. Also, Laeri et al showed that dye-loaded zeolite AlPO4-5 can function as microlaser. Only individual zeolite crystals with a dumbbelllike shape show laser emission.