Our experimental setup incorporated a Mettler Toledo EasyMax 102 synthesis workstation, equipped with an overhead stirrer and a SP-50 dosing unit for liquid handling. We opted for this commercialized ALR over custom or prototype SDL modules for its reliability, availability, and well-maintained user-friendly software families. We utilized the MT AutoChem software iControl 6.2 complemented by the iC Data Center 6.2 with Electronic Laboratory Notebook (ELN)-enabled capacity (detailed setup in ESI † section S4.2) to allow experiment design and automatic XML import from a designated folder. Once the LLM-generated XML file was moved to the folder, it should appear to the iControl ELN session if there was no syntax error (ESI † Fig. ). The experimental design interface in iControl can help visualize scripted operations, allowing easy fine-tuning. In case of any syntax error, the iC Data Center would create an error message file in the same folder that can be used to prompt the LLM for correction in the same dialogue (ESI † Fig. ). This error correction approach is similar that of CLAIRify, enabling GPT to correct the syntax error by understanding the error message.