Hybrid materials built from 2D monolayers are gaining attention as novel materials with potentially more easily tuneable properties. The current bottle-neck in exploiting these materials is the vast space of possible materials combinations, difficulty in predicting which will be best for a given application, and the real world experimental difficulties in synthesizing them. While electronic structure calculations can make these predictions accurately, even the most efficient methods DFT are too time-consuming to calculate the properties of every possible multilayer hybrid 2D material.