Additionally, we are able to produce the first large-scale and robust comparison of MC-PDFT to other single-reference methods such as CC2, and find the CASSCF mixing parameter of 0.25 used in tPBE0 to be optimal. We have made all the wave functions converged in this work available to the public via publication of the converged orbitals and CI vectors and encourage others to use these data in the development of further multireference model chemistries.