Applying dynamic operation to heterogeneous catalytic applications will require identifying the conditions of optimal performance in addition to new design variables such as surface waveform shape that can be implemented in real reactor technology. As depicted in Fig. , the sinusoidal surface binding waveform varying from -0.1 to +0.5 eV at frequency of 10 Hz applied to the catalyst system characterized by the volcano plot of Fig. yields oscillatory turnover frequency (Fig. ) and surface coverage of A* (Fig. ) at 100 bar A inlet, 150 °C, and 1% yield of B. Similar to the case with the square waveform, the turnover frequency of B increases when the applied waveform changes from strong binding of B* to weak binding. At the same time, the surface coverage of A* increases to take the place of the B* that was removed from the surface as desorbed product B. Other considered waveform types including triangle and sawtooth are depicted in Fig. . For all conditions, the square waveform exhibits superior activity at surface resonance conditions. At higher frequencies of 10 and 1,000 Hz, the sinusoidal waveform outperforms the triangle and sawtooth shapes.