However, to the best of our knowledge, no water model has been developed by adjusting the parameters to reproduce the surface tension directly; 25 in particular, water was not one of the four liquids studied in Ref. 23. The development of such a water model is needed for testing the hypothesis that surface tension can effectively substitute for the heat of vaporization in the force field parameterization. Moreover, the utility of surface tension as reference data for force field devleopment creates a need for automated tools and procedures that can effectively use this data to generate models for molecular liquids in systematic fashion.