We showed that AutoBADDIE is able to predict interatomic parameters that can drive MD simulations with performance matching those of parameterizations developed over decades of hand-tuning and scientific research such as OPLS and PCFF+. Across all systems investigated, including for those identical aside from different charge distributions on the TFSI, neither the force nor energy parity with respect to DFT were seen to be solely descriptive of an interatomic potential parameterization's ability to provide solvation or kinetic properties that match experimental measurements. The correct trend in conductivity across different salt concentrations was seen for the nitrogen-coordinating TFSI charges from DFT and the oxygen-coordinating TFSI charge distributions from DFT and by This