Alternative solvent suppression methods such as excitation sculpting and WATERGATE (WATER-suppression by GrAdient-Tailored Excitation, WG) retain signals from exchangeable nuclei, and do not require lengthy recovery delays. Instead, these methods use either selective pulses or binomial series of pulses, in combination with pulsed field gradients (PFGs), to refocus off-resonance solute signals while dephasing the on-resonance solute signal. Excitation sculpting has previously been integrated into the PSYCHE experiment; 11 however, that implementation provides poor solvent suppression. A WATERGATE pure shift method has also been reported in which WATERGATE was concatenated with the PSYCHE triple spin echo (TSE) experiment (W5n-TSE-PSYCHE where n represents the number of W5 elements). Although good solvent suppression has been reported with this method, the addition of separate WATERGATE elements causes unwanted scalar coupling evolution and leads to greatly increased chunking sidebands (see Supporting Information, Section E).