In conclusion, our Raman spectra of a large series of microporous carbons provide new evidence for disorder-driven capacitance. Nanoporous carbons with smaller ID/IG ratios and therefore smaller graphenelike domain sizes exhibited higher capacitances. This closely mirrors our previous findings where smaller graphene-like domain sizes measured with NMR spectroscopy and simulations also correlated with higher capacitances. Additionally, carbons with broader D bands, and thus a wider range of different carbon coherence lengths, also tended to have higher capacitance. Our study further shows that Raman