First, we find that the NPs aggregate inside the drop and localize inside the drop at locations that are closest to the magnet. This progressive aggregation can be noted from the constant brightening of the locations in the interior of the drop from where the NPs move away to form the nanoaggregates. A darker color of the drop interior suggests that there is the presence of the NPs; however, when the color of the drop interior at such locations becomes brighter, it indicates that a scarce number of NPs are present at such locations [see Figure ]. We also consider such aggregation of MNPs inside the MNLD and the subsequent nanoaggregate de-encapsulation for the MNLD created using a stronger aqueous dispersion of Fe3O4 [see Figure ]. For this case, one observes a faster aggregation and de-encapsulation (as can be noted from the corresponding timestamps). This aggregated mass of the NPs accumulates at the drop-PDMS interface at the location that is closest to the magnetic field. Subsequently, the presence of the magnetic field pulls the magnetic nanoaggregate downward and eventually the nanoaggregate gets completely extracted out of the drop with the drop itself retaining its spherical shape after the extraction [see Figure (b) and video M1]. Such pulling out of the MNPs or (MNP aggregates) from inside the drop in a manner such that the nanoaggregate gets completely detached from the drop and the drop remains intact, represents a most unique and remarkable situation where there is an almost complete deencapsulation of the aggregated particles from the interior of a drop. Very often particles localize at the drop-air or drop-liquid interface , but never completely de-encapsulates from the drop, typically stemming from the very large capillary forces that these particles must overcome for completely breaching the interface. In the present case, however, a large magnetic force acts on the nanoaggregates -this high magnetic force stems from a combination of the MNPs forming an aggregate, i.e., creating a highly concentrated zone of the MNPs, and the presence of a strong magnetic field -and enables the aggregate to overcome the restraining capillary force exerted by the drop-PDMS interface. To the best of our knowledge, this is the first study that shows such deencapsulation of particles from the interior of a liquid drop.