To succinctly characterize the germanium distribution for each zeolite framework across a broad range of Si/Ge ratios in more detail (Figures and), we focus below only on a few descriptors, : i) the relative occupations of various classes of T-sites (D4R, framework and adjacent -see Section 2 and SI Figure for definition), ii) the relative occupations of each individual D4R unit in the unit cell: representing asymmetry in D4R occupations, iii) the global structure optima (GSO) for the germanium loading at specific Ge loadings. Further relevant characterizations, e.g., a broader set of low-energy structures, will be only briefly discussed, with the details provided in the Supporting Information.