The frozen energy can be further decomposed into contributions from frozen electrostatics E elec , dispersion E disp , and Pauli repulsion E Pauli . Electrostatic energies are computed similarly to equation 7, but with the actual DFT densities between each fragment. Dispersion energies are computed by subtracting out a "dispersion-free" contribution from the frozen XC energy using distorted fragment density matrices. The remaining frozen contribution is thus attributed to Pauli repulsion (E Pauli = E frz -E elec -E disp ) results from the orthogonalization of molecular orbitals being brought in from infinity. This procedure is similar to that used in Demerdash et al . The polarization energy is computed as the additional energy relaxation of the total electronic system under the absolutely localized molecular orbital (ALMO) anzatz. Here, E pol constitutes the contribution to E int resulting from simply responding to the presence of another nearby fragment, but under the constraint that each fragment's molecular orbitals can only be constructed from their respective atomic orbitals. Therefore, fitting our model directly to this energy incorporates both electrostatic contributions to polarization, as well as all energetic costs due to kinetic and XC energies. As molecular polarizability (or inversely, molecular hardness) involves all such contributions, EDA polarization energy is an appropriate quantity to fit our model polarization energy against. Lastly, the charge transfer contributions E ct makes up the remaining interaction energy resulting from a fully (counterpoise corrected) relaxed molecular system using all atomic orbitals from all fragments. To summarize,