Figures 3c shows that the ohmic resistance, charge-transfer resistance, and polarization resistance are all dominated by a key peak frequency of the dynamic discharge current profile (f2 in Figure ), as well as the maximum instantaneous discharge current. These discharge current frequencies are all well below 1 Hz (ranging from 0.05 to 64 mHz), corresponding to Faradaic processes. We hypothesize that these correlations may be due to differences in electrode particle activation at higher frequencies and reduced local stresses and heterogeneities at low frequencies . Additionally, the electrode-specific capacities, obtained using a half-cell differential voltage model (see Methods) display distinct correlations with dynamic discharge features. First, the negative electrode (anode) degradation is dictated by the maximum instantaneous discharge current and the current variance. The combination of resistance growth and large discharge current peaks (which can reach up to 1800 % of the average C-rate in synthetic and real driving protocols) gives rise to larger overpotentials.