Many chiral helicenes show interesting chiroptical properties and these materials have been widely investigated in such diverse fields as bioimaging, optical data storage, optical spintronics applications, and circularly polarized organic light-emitting diodes (CP-OLEDs). Most emissive chiral helicenes are fluorescent, but for efficient OLEDs, triplet excitons need to be harvested, so helicenes that emit either phosphorescence or thermally activated delayed fluorescence (TADF) would be potentially attractive emitters. Organic multi-resonant TADF (MR-TADF) materials have attracted particular attention as emitters for OLEDs as not only can devices attain 100% internal quantum efficiency (IQE) but they also show narrowband emission and high photoluminescence quantum yield (FPL). Thus, the development of chiral MR-TADF emitters would be particularly attractive for CP-MR-TADF OLEDs.