In the original ALMO-CIS/TDA formalism, fragment indices X = Y is enforced in Eq. ( ) such that the full-system excitations are represented as the superposition of many absolutely localized on-fragment excitations. An extension that incorporates charge-transfer excitations to or from nearby fragments was proposed later. Here we employ a fully generalized version of this method: taking advantage of the fragment tags of occupied and virtual orbitals, one can include each fragment's occupied and/or virtual orbitals in the active space for single excitations. In the end, the amplitudes t XiYa may include a mixture of on-fragment and interfragment occupied→virtual transitions. This generalized ALMO-TDA scheme, which has been implemented in the Q-Chem software package, allow us to shed light on the orbital entanglement effects from an alternative perspective.