Although a large number of topologically distinct framework types are available in high-silica or even all-silica form, the structural diversity of zeolites in terms of pore size and pore topology has hardly been explored in the context of CE adsorption. The present study aims to fill this gap, employing a combination of Henry constant simulations and GCMC simulations to study the adsorption of all species listed in Table in 16 all-silica zeolites. These particular frameworks were selected for the following reasons: (1) They can by synthesized in pure-silica or high-silica form. (2) They possess different pores sizes and connectivities. (3) According to preliminary simulations, described below, their pore apertures are large enough to permit the diffusion of all CE molecules. Through GCMC simulations for very low partial pressures, conclusions regarding the potential suitability of zeolites to remove trace amounts (down to sub-ppm range) of CEs are drawn. Moreover, a closer look is taken at simulation snapshots in order to elucidate the microscopic origins of the observed affinities of selected frameworks.