As the dynamics restart from the reset wave function, the PES used in the propagation is slowly updated from the PES before the new SPs were added to the new PES obtained using the new SPs, in the interval [1800, 1900] a.u. Fig. shows the final TD-ADGA iteration where new SPs are added. This iteration is carried out after a time-propagation of 14900 a.u. A restart similar to the one described for Fig. is then carried out. After this restart, the PES is considered converged for the rest of the dynamics simulation and no more SPs are added.