Our focus is on generating extensive and complete numerical data, aimed at enhancing future scientific research in the field of ML-assisted design of solid solution alloys with desired thermodynamic and mechanical functional properties. Our data collection process has been used to to perform VASP calculations on a total of 19,800 atomic configurations across all binaries and ternaries, collectively amounting to approximately 120,000 compute node hours on OLCF-Summit and 100,000 node hours on NERSC-Perlmutter. For each configuration, we launched concurrent VASP computations using multiple GPUs distributed across multiple nodes on both supercomputing facilities.