Classical molecular dynamics (CMD) calculations are a typical atomic simulation technique for structural analysis and can be used to evaluate the three-dimensional structure of a glass, including its atomic dynamics. However, the accuracy of the results obtained with CMD is strongly dependent on the potential parameters used. Although many CMD modeling studies of multicomponent glasses have been reported, there are limited available potential parameters that can enable reproduction of experimental data for a wide variety of glass compositions. The potential parameters developed by Wang et al. and Deng and Du (referred to as CMD-Wang and CMD-Du, respectively, hereafter) are known to be highly accurate for multicomponent glass systems, including aluminoborosilicate-containing group 1 and 2 cations. CMD-Du has also been used to successfully reproduce the specific behavior of the four-coordinate boron (B 4 ) population with increasing alkali metal content.