To expand the developed organocatalytic process toward the construction of spiro compounds containing 3-, 4-, and 6membered rings (Scheme 3), 1-bromonitroalkanes 2 with various lengths of alkyl moiety were subjected to the reaction with methyleneindolinone 1a. With respect to previously reported methods, 17 we isolated corresponding spirooxindolefused cyclopropane 6 in good yield and stereochemical outcomes. Despite known examples of spirooxindole-fused cyclobutanes, 11b we did not observe any conversion of starting methyleneindolinone 1a in reaction with 1-bromo-2nitroethane (2c). Interestingly, reaction of longer 1-bromo-2nitrobutane produced unseparable complex mixture of products with major uncyclized products of the Michael reaction.