Molecular dynamics (MD) has received considerable attention in polymer and biopolymer research as a computational tool to describe the ensemble and time-dependent behavior of atomistically detailed molecular systems. Software for classical MD utilizes force fields, which describe the potential energy and forces on atoms in a chemical topology, to integrate the dynamics of a system over time via numerical integration of Newton's equations of motion. These force fields generally consist of parameters that describe the atomic valence (bond stretch, angle, and dihedral) and non-bonded (electrostatic and van der Waals) forces, resulting in molecular ensembles useful for predicting thermophysical properties of many systems and providing mechanistic insight useful to experimental research and engineering.