In conclusion, functionalized supramolecular noodles can be used as templates for spatially resolved photopolymerization. We have shown that new photoinitiators can be produced and tailored to retain the self-assembly gelation properties of micellar dipeptides. Furthermore, by modifying the linker group between the benzophenone-based photoinitiator component and the dipeptide component, the viscosity can be sufficiently increased to enable supramolecular noodle formation. The noodles are robust enough to be manually handled for pattern templating, and their mechanical properties remain unaffected after annealing their micellar solutions. Photopolymerization of a cross-linkable acrylate monomer around the shell of the noodle can yield structures that are rigid and exhibit significantly increased mechanical strength. Alternatively, mono-acrylate monomers can be used to produce softer yet still self-supporting structures that do not dissolve in common organic solvents. We have also shown that our system of templating can be used to create more structurally complex materials. By tailoring the polymerisation time to suit the monomer, we can produce shapes containing details that are difficult to mimic without complex instrumentation or experimental setups, such as hollow tubes and sections that intersect.