We assessed the ability of molecular dynamics simulations using the newly fitted Parsley force field to replicate 221 experimental observables for organic liquids spanning 104 molecules. The observables used are densities, heats of vaporization, and static dielectric constants, of pure liquids, and excess molar volumes and heats of mixing of binary liquid mixtures. The experimental data were drawn from the NIST ThermoML Archive. For systems involving water, the TIP3P model was used. Automated scripts used to select the data can be found in Supporting Information section 1.2.2.