 Nyorai kupfuurira kweiyi ndima - Jolie akatsigirawo dzidzo yevana. Kubvira payakatangwa pamusangano wepagore weClinton Global Initiative munaGunyana 2007, ave achitungamira Education Partnership for Children of Conflict, iyo inopa mutemo uye mari yezvirongwa zvedzidzo zvevana mumatunhu akakanganiswa nemhirizhonga. Mugore rayo rokutanga, kudyidzana kwakatsigira mapurojekiti edzidzo kuvana vevapoteri veIraq, vechidiki vakakanganiswa nekunetsana kweDarfur, uye vasikana mumaruwa eAfghanistan, pakati pemamwe mapoka akabatwa. Kubatana uku kwakashanda pamwe chete neCentre for Universal Education yeCouncil on Foreign Relations, iyo yakavambwa nemumwe wemutungamiri wekubatana uku, nyanzvi yezvehupfumi Gene Sperling, kuti vagadzire marongero edzidzo, izvo zvakakonzera kurudziro dzakaitwa kumasangano eUN, masangano ekuvandudza eG8, neWorld Bank. Kubva muna Kubvumbi 2013, mari yese kubva kuJolies high-end jewelry collection, Style of Jolie, yakabatsira basa rekudyidzana. Jolie zvakare akatanga Malala Fund, hurongwa hwekubatsira hwakagadzwa nePakistani mudzidzi wezvedzidzo Malala Yousafzai, ku2013 Women in the World Summit; iye pachake akapa mari inodarika 200,000 kuchinangwa. 